2023Journal Article ER4 Auteurs : Billmann, Madeleine; Hulot, Corinne; Pauget, Benjamin; Badreddine, Rabia; Papin, Arnaud; Pelfrêne, Aurélie Oral bioaccessibility of PTEs in soils: A review of data, influencing factors and application in human health risk assessment In: Science of the Total Environment, vol. 896, pp. 165263, 2023, (ACL). Links @article{billmann:hal-04288865,
title = {Oral bioaccessibility of PTEs in soils: A review of data, influencing factors and application in human health risk assessment},
author = {Madeleine Billmann and Corinne Hulot and Benjamin Pauget and Rabia Badreddine and Arnaud Papin and Aurélie Pelfrêne},
url = {https://hal.science/hal-04288865},
doi = {10.1016/j.scitotenv.2023.165263},
year = {2023},
date = {2023-10-01},
urldate = {2023-10-01},
journal = {Science of the Total Environment},
volume = {896},
pages = {165263},
publisher = {Elsevier},
note = {ACL},
keywords = {ER4},
pubstate = {published},
tppubtype = {article}
}
|
2022Conference ER4 Auteurs : Cheval, Pénélope; Vandoorne, Bertrand; Douay, Francis; Pruvot, Christelle; Pelfrêne, Aurélie Construction of functional and fertile Technosols from materials,
waste and by-products for use in biointensive micro-gardening Soil Science, Crossing Boundaries, Changing Society (22 WCSS), 31
July-5August 2022, Glasgow (Scotland, United Kingdom), 2022, (ACTI). Abstract @conference{Cheval2022,
title = {Construction of functional and fertile Technosols from materials,
waste and by-products for use in biointensive micro-gardening},
author = {Pénélope Cheval and Bertrand Vandoorne and Francis Douay and Christelle Pruvot and Aurélie Pelfrêne},
year = {2022},
date = {2022-01-01},
booktitle = {Soil Science, Crossing Boundaries, Changing Society (22 WCSS), 31
July-5August 2022, Glasgow (Scotland, United Kingdom)},
abstract = {Soil is a limited resource subject to multiple pressures. Soil degradation sometimes leads to the loss of its functions, which is an irreversible process on a lifetime scale. The area covered by fertile soil decreases as it is exposed to anthropogenic activities. To meet the demand for the reconnection to food production in cities, it appears interesting to conceive functional Technosols using materials, waste, and by-products instead of extracting and transporting natural fertile soils. Technosols are soils with at least 20% of artifacts, a geomembrane or a technic hard rock. In the present work, two Technosols were designed and tested in a greenhouse experiment for a bio-intensive micro-gardening use. Their conception was based on the physico-chemical characteristics of soils known for their high agronomic potential for vegetable growing, as well as on the selection of available materials whose characteristics met the expectations. For one year, three aspects were studied to assess the ability of Technosols to support the production of food biomass. These include the pedological component by measuring the physico-chemical parameters of the Technosols; the biological component comprising several bio-indicator organisms of the soil fauna as well as ecophysiological indicators of the crops (photosynthetic and nitrogenous status) and their development; and the ecological engineering component by studying the ability of an ecosystem engineers to improve the fertility of the Technosols. After a few months, some pedogenetic processes were initiated and the indicators selected to evaluate the fertility of the constructed Technosols showed a good potential to support vegetable crops.},
note = {ACTI},
keywords = {ER4},
pubstate = {published},
tppubtype = {conference}
}
Soil is a limited resource subject to multiple pressures. Soil degradation sometimes leads to the loss of its functions, which is an irreversible process on a lifetime scale. The area covered by fertile soil decreases as it is exposed to anthropogenic activities. To meet the demand for the reconnection to food production in cities, it appears interesting to conceive functional Technosols using materials, waste, and by-products instead of extracting and transporting natural fertile soils. Technosols are soils with at least 20% of artifacts, a geomembrane or a technic hard rock. In the present work, two Technosols were designed and tested in a greenhouse experiment for a bio-intensive micro-gardening use. Their conception was based on the physico-chemical characteristics of soils known for their high agronomic potential for vegetable growing, as well as on the selection of available materials whose characteristics met the expectations. For one year, three aspects were studied to assess the ability of Technosols to support the production of food biomass. These include the pedological component by measuring the physico-chemical parameters of the Technosols; the biological component comprising several bio-indicator organisms of the soil fauna as well as ecophysiological indicators of the crops (photosynthetic and nitrogenous status) and their development; and the ecological engineering component by studying the ability of an ecosystem engineers to improve the fertility of the Technosols. After a few months, some pedogenetic processes were initiated and the indicators selected to evaluate the fertility of the constructed Technosols showed a good potential to support vegetable crops. |
2022Conference ER4 Auteurs : Cheval, Pénélope; Vandoorne, Bertrand; Douay, Francis; Pruvot, Christelle; Pelfrêne, Aurélie Using constructed Technosols for urban bio-intensive market gardening:
assessment of their habitat and food biomass production function 11th Conference on Soils of Urban, Industrial, Traffic and Mining
Areas (SUITMA), 5-9 September 2022, Berlin (Germany), 2022, (ACTI). Abstract @conference{Cheval2022a,
title = {Using constructed Technosols for urban bio-intensive market gardening:
assessment of their habitat and food biomass production function},
author = {Pénélope Cheval and Bertrand Vandoorne and Francis Douay and Christelle Pruvot and Aurélie Pelfrêne},
year = {2022},
date = {2022-01-01},
booktitle = {11th Conference on Soils of Urban, Industrial, Traffic and Mining
Areas (SUITMA), 5-9 September 2022, Berlin (Germany)},
abstract = {Soil is an essential component of terrestrial ecosystems as it provides many functions and ecosystem services. Soil is the product of various physical, chemical, and biological processes that take place over thousands to millions of years. As a result, soil is a non-renewable resource on a human lifetime scale. In urban areas, soil undergoes many anthropogenic pressures resulting from land development, which sometimes leads to a degradation of its quality along with a partial or total loss of its functions and ecosystem services. Consequently, the areas covered by fertile soils in urban and peri-urban environments are decreasing as they are reclaimed. Urban land-use policy is evolving and aims to enhance projects that reconnect food production in urban areas. As cities have available unused materials, wastes and by-products, it seems interesting to consider using them for the conception of Technosols for urban vegetable production. Technosols are soils with at least 20% of artifacts, a geomembrane, or a technic hard rock. In the present work, two constructed Technosols were designed and tested in a greenhouse experiment for market gardening. Their conception was based on the physico-chemical characteristics of soils known for their high agronomic potential for vegetable growing, as well as on the selection of available materials whose characteristics met the expectations (e.g., uncontaminated materials, locally available and sustainably supplied). During a one-year period, three aspects were studied to evaluate the capacity of the Technosols to ensure habitat (for specific soil fauna organisms selected regarding their ability to be suitable indicators of the quality of their environment) and food biomass production functions. First, the pedological component was examined by measuring the physico-chemical parameters of the Technosols; secondly the study focused on the characterization of the biological component, comprising several bio-indicator organisms of the soil fauna as well as eco-physiological indicators of the crops (photosynthetic and nitrogenous status) and their development; finally, the ecological engineering component was analyzed by studying the ability of an ecosystem engineer (Lumbricus terrestris) to improve the fertility of the Technosols. After a few months, some pedogenetic processes were initiated (e.g., settlement, weathering of parent materials) and the indicators selected to evaluate the fertility of the constructed Technosols (physico-chemical and biological parameters) showed a good potential to support vegetable crops. Upon establishment of the constructed Technosols, some of the selected soil fauna bioindicators were also able to sustain their fitness, suggesting the initiation of a future trophic web.},
note = {ACTI},
keywords = {ER4},
pubstate = {published},
tppubtype = {conference}
}
Soil is an essential component of terrestrial ecosystems as it provides many functions and ecosystem services. Soil is the product of various physical, chemical, and biological processes that take place over thousands to millions of years. As a result, soil is a non-renewable resource on a human lifetime scale. In urban areas, soil undergoes many anthropogenic pressures resulting from land development, which sometimes leads to a degradation of its quality along with a partial or total loss of its functions and ecosystem services. Consequently, the areas covered by fertile soils in urban and peri-urban environments are decreasing as they are reclaimed. Urban land-use policy is evolving and aims to enhance projects that reconnect food production in urban areas. As cities have available unused materials, wastes and by-products, it seems interesting to consider using them for the conception of Technosols for urban vegetable production. Technosols are soils with at least 20% of artifacts, a geomembrane, or a technic hard rock. In the present work, two constructed Technosols were designed and tested in a greenhouse experiment for market gardening. Their conception was based on the physico-chemical characteristics of soils known for their high agronomic potential for vegetable growing, as well as on the selection of available materials whose characteristics met the expectations (e.g., uncontaminated materials, locally available and sustainably supplied). During a one-year period, three aspects were studied to evaluate the capacity of the Technosols to ensure habitat (for specific soil fauna organisms selected regarding their ability to be suitable indicators of the quality of their environment) and food biomass production functions. First, the pedological component was examined by measuring the physico-chemical parameters of the Technosols; secondly the study focused on the characterization of the biological component, comprising several bio-indicator organisms of the soil fauna as well as eco-physiological indicators of the crops (photosynthetic and nitrogenous status) and their development; finally, the ecological engineering component was analyzed by studying the ability of an ecosystem engineer (Lumbricus terrestris) to improve the fertility of the Technosols. After a few months, some pedogenetic processes were initiated (e.g., settlement, weathering of parent materials) and the indicators selected to evaluate the fertility of the constructed Technosols (physico-chemical and biological parameters) showed a good potential to support vegetable crops. Upon establishment of the constructed Technosols, some of the selected soil fauna bioindicators were also able to sustain their fitness, suggesting the initiation of a future trophic web. |
2022Conference ER4 Auteurs : Pelfrêne, Aurélie Bioaccessibilité des polluants : Apport à l’évaluation de l’exposition
des populations vivant sur des sites contaminés Cérémonie d’entrée des nouveaux associés de la SCIC Crisalid, 31
mai 2022, 2022, (COM). @conference{Pelfrene2022,
title = {Bioaccessibilité des polluants : Apport à l’évaluation de l’exposition
des populations vivant sur des sites contaminés},
author = {Aurélie Pelfrêne},
year = {2022},
date = {2022-01-01},
booktitle = {Cérémonie d’entrée des nouveaux associés de la SCIC Crisalid, 31
mai 2022},
note = {COM},
keywords = {ER4},
pubstate = {published},
tppubtype = {conference}
}
|
2022Conference ER4 Auteurs : Schnackenberg, Ashley; Bidar, Géraldine; Bert, Valérie; Cannavo, Patrice; Détriché, Sébastien; Douay, Francis; Guenon, René; Jean-Soro, Liliane; Kohli, Alice; Lebeau, Thierry; Perronnet, Karen; Vidal-Beaudet, Laure; Waterlot, Christophe; Pelfrêne, Aurélie Effects of amendments on the mobility, bioaccessibility, and phytoavailability of As, Cd, Pb, and Zn in contaminated urban kitchen garden soils 11th Conference on Soils of Urban, Industrial, Traffic and Mining Areas (SUITMA), 5-9 September 2022, Berlin (Germany), 2022, (ACTI). Abstract @conference{Schnackenberg2022,
title = {Effects of amendments on the mobility, bioaccessibility, and phytoavailability of As, Cd, Pb, and Zn in contaminated urban kitchen garden soils},
author = {Ashley Schnackenberg and Géraldine Bidar and Valérie Bert and Patrice Cannavo and Sébastien Détriché and Francis Douay and René Guenon and Liliane Jean-Soro and Alice Kohli and Thierry Lebeau and Karen Perronnet and Laure Vidal-Beaudet and Christophe Waterlot and Aurélie Pelfrêne},
year = {2022},
date = {2022-01-01},
booktitle = {11th Conference on Soils of Urban, Industrial, Traffic and Mining Areas (SUITMA), 5-9 September 2022, Berlin (Germany)},
abstract = {Urban gardening is a growing trend that responds to the need for nature in cities, a growing movement towards healthy and sustainable eating and food production, and difficult economic and societal contexts. Both private and community gardens in these areas are often on urban wastelands, along roads, highways, or railways, near industrial sites, and have even sometimes earned the term “guerrilla gardens” for their lack of agronomic regulation. In France, many urban gardens are associated with varying levels of inorganic contaminants hailing from anthropogenic activity or geogenic metal(loid) presence. Moderately metal(loid)- contaminated urban kitchen garden soils can benefit from gentle remediation options including the use of soil amendments, which are able to improve soil function and agronomic quality while decreasing environmental and human health risk. This study first analyses the effects of common doses of a various commercialized soil amendments on the mobility of metalloid(s) in contaminated urban kitchen garden soils. Fourteen different amendments and amendment mixes were tested on three kitchen garden soils with diverse sources of anthropogenic or geogenous contamination and varying physico-chemical characteristics. Amendments from four differing categories were tested, including i) organic amendments like composts, ii) natural fertilizers such as bone meal, crushed horn, and organic poultry manure fertilizer, iii) calcareous amendments including two different limes, and iv) natural siliceous and alumino-silicate amendments, including diatomaceous earth and zeolite. Amendments at varying common doses were evaluated via chemical extractions on their ability to reduce the mobility of metallic elements after multiple weeks of maturation at a constant humidity and temperature. The most pertinent of these amendments were then chosen to be tested in conjunction with a vegetal model grown upon the amended soils in greenhouse conditions. 05.09.– 09.09 2022 Berlin, Germany Changes in physico-chemical soil characteristics, mobility and bioaccessibility of metal(loid)s in the soil, and phytoavailability in the lettuce were then tested. Mobility and bioaccessible metal(loid)s were evaluated with 0.05 M EDTA buffered at a pH of 7, an ammonium nitrate extraction, a 4-phase sequential extraction, and a UBM bioaccessibility test. Phytoavailability was determined using pseudo-total soil and plant metal(loid) contents. The study results show that it is possible to reduce both extractable and phytoavailable metal(oid)s with amendment addition. However, variable effects are seen according to the contaminated soil tested, and differences arise in the presence of a plant model.},
note = {ACTI},
keywords = {ER4},
pubstate = {published},
tppubtype = {conference}
}
Urban gardening is a growing trend that responds to the need for nature in cities, a growing movement towards healthy and sustainable eating and food production, and difficult economic and societal contexts. Both private and community gardens in these areas are often on urban wastelands, along roads, highways, or railways, near industrial sites, and have even sometimes earned the term “guerrilla gardens” for their lack of agronomic regulation. In France, many urban gardens are associated with varying levels of inorganic contaminants hailing from anthropogenic activity or geogenic metal(loid) presence. Moderately metal(loid)- contaminated urban kitchen garden soils can benefit from gentle remediation options including the use of soil amendments, which are able to improve soil function and agronomic quality while decreasing environmental and human health risk. This study first analyses the effects of common doses of a various commercialized soil amendments on the mobility of metalloid(s) in contaminated urban kitchen garden soils. Fourteen different amendments and amendment mixes were tested on three kitchen garden soils with diverse sources of anthropogenic or geogenous contamination and varying physico-chemical characteristics. Amendments from four differing categories were tested, including i) organic amendments like composts, ii) natural fertilizers such as bone meal, crushed horn, and organic poultry manure fertilizer, iii) calcareous amendments including two different limes, and iv) natural siliceous and alumino-silicate amendments, including diatomaceous earth and zeolite. Amendments at varying common doses were evaluated via chemical extractions on their ability to reduce the mobility of metallic elements after multiple weeks of maturation at a constant humidity and temperature. The most pertinent of these amendments were then chosen to be tested in conjunction with a vegetal model grown upon the amended soils in greenhouse conditions. 05.09.– 09.09 2022 Berlin, Germany Changes in physico-chemical soil characteristics, mobility and bioaccessibility of metal(loid)s in the soil, and phytoavailability in the lettuce were then tested. Mobility and bioaccessible metal(loid)s were evaluated with 0.05 M EDTA buffered at a pH of 7, an ammonium nitrate extraction, a 4-phase sequential extraction, and a UBM bioaccessibility test. Phytoavailability was determined using pseudo-total soil and plant metal(loid) contents. The study results show that it is possible to reduce both extractable and phytoavailable metal(oid)s with amendment addition. However, variable effects are seen according to the contaminated soil tested, and differences arise in the presence of a plant model. |
2022Journal Article ER4 Auteurs : Schnackenberg, Ashley; Bidar, Géraldine; Bert, Valérie; Cannavo, Patrice; Détriché, Sébastien; Douay, Francis; Guenon, René; Jean-Soro, Liliane; Kohli, Alice; Lebeau, Thierry; Perronnet, Karen; Vidal-Beaudet, Laure; Waterlot, Christophe; Pelfrêne, Aurélie Effects of Inorganic and Organic Amendments on the Predicted Bioavailability of As, Cd, Pb and Zn in Kitchen Garden Soils In: Advances in Environmental and Engineering Research, vol. 3, pp. 1 - 1, 2022, (ACL). Links @article{schnackenberg:hal-03583334,
title = {Effects of Inorganic and Organic Amendments on the Predicted Bioavailability of As, Cd, Pb and Zn in Kitchen Garden Soils},
author = {Ashley Schnackenberg and Géraldine Bidar and Valérie Bert and Patrice Cannavo and Sébastien Détriché and Francis Douay and René Guenon and Liliane Jean-Soro and Alice Kohli and Thierry Lebeau and Karen Perronnet and Laure Vidal-Beaudet and Christophe Waterlot and Aurélie Pelfrêne},
url = {https://hal.archives-ouvertes.fr/hal-03583334},
doi = {10.21926/aeer.2201004},
year = {2022},
date = {2022-02-01},
urldate = {2022-02-01},
journal = {Advances in Environmental and Engineering Research},
volume = {3},
pages = {1 - 1},
note = {ACL},
keywords = {ER4},
pubstate = {published},
tppubtype = {article}
}
|
2021Journal Article ER4 Auteurs : Glorennec, Philippe; Shendell, Derek-G.; Rasmussen, Pate E; Waeber, Roger; Egeghy, Peter; Azuma, Kenichi; Pelfrêne, Aurélie; Le-Bot, Barbara; Esteve, Williams; Perouel, Guillaume; Pernelet-Joly, Valérie; Noack, Yves; Delannoy, Matthieu; Keirsbulck, Marion; Mandin, Corinne Towards setting public health guidelines for chemicals in indoor settled dust? In: Indoor Air, vol. 31, no. 1, pp. 112-115, 2021, (ACL). Abstract @article{Glorennec2021,
title = {Towards setting public health guidelines for chemicals in indoor settled dust?},
author = {Philippe Glorennec and Derek-G. Shendell and Pate E Rasmussen and Roger Waeber and Peter Egeghy and Kenichi Azuma and Aurélie Pelfrêne and Barbara Le-Bot and Williams Esteve and Guillaume Perouel and Valérie Pernelet-Joly and Yves Noack and Matthieu Delannoy and Marion Keirsbulck and Corinne Mandin},
year = {2021},
date = {2021-01-01},
journal = {Indoor Air},
volume = {31},
number = {1},
pages = {112-115},
abstract = {Indoor settled dust may result in substantial human exposure to chemicals,
especially by ingestion following hand‐to‐mouth or hand‐to‐object‐to‐mouth
contact. As with other environmental media related to exposure, dust
may thus be subject to regulation. An international scientific workshop
was convened in Paris in September 2019firstly to assess the relevance
for public health of setting guidelines for indoor settled dust,
and secondly to discuss scientific and technical challenges related
to such guidelines. The main discussions and conclusions, with consensus
achieved, are reported herein. Discussions concernedgeneral considerations,objectives
and definitions, relevance for a health‐based guideline, units of
measure, and finally derivation of the guideline.These points should
be addressed when consideringan indoor settled dust guideline as
part of a policy to reduce exposure indoors to a given chemical or
group of chemicals.},
note = {ACL},
keywords = {ER4},
pubstate = {published},
tppubtype = {article}
}
Indoor settled dust may result in substantial human exposure to chemicals,
especially by ingestion following hand‐to‐mouth or hand‐to‐object‐to‐mouth
contact. As with other environmental media related to exposure, dust
may thus be subject to regulation. An international scientific workshop
was convened in Paris in September 2019firstly to assess the relevance
for public health of setting guidelines for indoor settled dust,
and secondly to discuss scientific and technical challenges related
to such guidelines. The main discussions and conclusions, with consensus
achieved, are reported herein. Discussions concernedgeneral considerations,objectives
and definitions, relevance for a health‐based guideline, units of
measure, and finally derivation of the guideline.These points should
be addressed when consideringan indoor settled dust guideline as
part of a policy to reduce exposure indoors to a given chemical or
group of chemicals. |
2021Journal Article ER4 Auteurs : Perouel, Guillaume; Keirsbulck, Marion; Chaigneau, Thomas; Delannoy, Matthieu; Esteve, Williams; Bot, Barbara Le; Noack, Yves; Pelfrêne, Aurélie; Glorennec, Philippe Exposure assessment and reference values for settled dust in indoor environments In: Environnement Risques Santé, vol. 20, no. 4, pp. 383–388, 2021. Links @article{Perouel2021,
title = {Exposure assessment and reference values for settled dust in indoor environments},
author = {Guillaume Perouel and Marion Keirsbulck and Thomas Chaigneau and Matthieu Delannoy and Williams Esteve and Barbara Le Bot and Yves Noack and Aurélie Pelfrêne and Philippe Glorennec},
doi = {10.1684/ers.2021.1569},
year = {2021},
date = {2021-08-01},
journal = {Environnement Risques Santé},
volume = {20},
number = {4},
pages = {383--388},
publisher = {John Libbey Eurotext},
keywords = {ER4},
pubstate = {published},
tppubtype = {article}
}
|
2021Journal Article ER4 Auteurs : Louzon, Maxime; Pauget, Benjamin; Pelfrêne, Aurélie; Gimbert, Frédéric; Vaufleury, Anette Combining human and snail indicators for an integrative risk assessment of metal(loid)-contaminated soils In: Journal of Hazardous Materials, vol. 409, pp. 124182, 2021, ISSN: 0304-3894, (ACL). Abstract | Links @article{LOUZON2021124182,
title = {Combining human and snail indicators for an integrative risk assessment of metal(loid)-contaminated soils},
author = {Maxime Louzon and Benjamin Pauget and Aurélie Pelfrêne and Frédéric Gimbert and Anette Vaufleury },
url = {https://www.sciencedirect.com/science/article/pii/S0304389420321725},
doi = {https://doi.org/10.1016/j.jhazmat.2020.124182},
issn = {0304-3894},
year = {2021},
date = {2021-01-01},
urldate = {2021-01-01},
journal = {Journal of Hazardous Materials},
volume = {409},
pages = {124182},
abstract = {With the new soil uses such as land restoration and to protect wilderness, the human health risk assessment (HHRA) and environmental risk assessment (ERA) should be combined. Based on the relationships demonstrated between an indicator of soil quality, the land snail, and human exposure, the aim of this study is to examine the snail and human risk indicators for twenty-nine soils contaminated by metal(loid)s. HHRA was evaluated by both hazard quotient and carcinogenic risk. When the human health indicators were ranked as uncertain, they were weighted by bioaccessibility to refine the risk assessment. The ERA was performed with risk coefficient after ex situ snail exposure. The results showed strong and novel relationships between human health and environmental risk indicators that had never been found before. For 62% of the soils, both indicators revealed either a confirmed risk or an uncertain level of risk. Overall pollutants present greater risk for human than for environment, with 55 vs 28% of the studied soils classified in the proven risk, respectively. An original integrative risk assessment of polluted soils has been proposed, that shall help setting up relevant strategies to manage contaminated soils considering not only human but also environmental indicators of risk.},
note = {ACL},
keywords = {ER4},
pubstate = {published},
tppubtype = {article}
}
With the new soil uses such as land restoration and to protect wilderness, the human health risk assessment (HHRA) and environmental risk assessment (ERA) should be combined. Based on the relationships demonstrated between an indicator of soil quality, the land snail, and human exposure, the aim of this study is to examine the snail and human risk indicators for twenty-nine soils contaminated by metal(loid)s. HHRA was evaluated by both hazard quotient and carcinogenic risk. When the human health indicators were ranked as uncertain, they were weighted by bioaccessibility to refine the risk assessment. The ERA was performed with risk coefficient after ex situ snail exposure. The results showed strong and novel relationships between human health and environmental risk indicators that had never been found before. For 62% of the soils, both indicators revealed either a confirmed risk or an uncertain level of risk. Overall pollutants present greater risk for human than for environment, with 55 vs 28% of the studied soils classified in the proven risk, respectively. An original integrative risk assessment of polluted soils has been proposed, that shall help setting up relevant strategies to manage contaminated soils considering not only human but also environmental indicators of risk. |
2021Journal Article ER4 Auteurs : Nsanganwimana, Florien; Souki, Karim Suhail Al; Waterlot, Christophe; Douay, Francis; Pelfrêne, Aurélie; Ridošková, Andrea; Louvel, Brice; Pourrut, Bertrand Potentials of Miscanthus x giganteus for phytostabilization of trace element-contaminated soils: Ex situ experiment In: Ecotoxicology and Environmental Safety, vol. 214, pp. 112125, 2021, ISSN: 0147-6513, (ACL). Abstract | Links @article{NSANGANWIMANA2021112125,
title = {Potentials of Miscanthus x giganteus for phytostabilization of trace element-contaminated soils: Ex situ experiment},
author = {Florien Nsanganwimana and Karim Suhail Al Souki and Christophe Waterlot and Francis Douay and Aurélie Pelfrêne and Andrea Ridošková and Brice Louvel and Bertrand Pourrut},
url = {https://www.sciencedirect.com/science/article/pii/S0147651321002360},
doi = {https://doi.org/10.1016/j.ecoenv.2021.112125},
issn = {0147-6513},
year = {2021},
date = {2021-01-01},
urldate = {2021-01-01},
journal = {Ecotoxicology and Environmental Safety},
volume = {214},
pages = {112125},
abstract = {Phytomanagement is proposed as a cost-effective and environmentally-friendly suggestion for sustainable use of large metal-contaminated areas. In the current work, the energy crop miscanthus (Miscanthus × giganteus) was grown in ex situ conditions on agricultural soils presenting a Cd, Pb and Zn contamination gradient. After 93 days of culture, shoot and root growth parameters were measured. Soils and plants were sampled as well to study the TE accumulation in miscanthus and the effects of this plant on TE mobility in soils. Results demonstrated that miscanthus growth depended more on the soils silt content rather than TE-contamination level. Moreover, soil organic carbon at T93 increased in the soils after miscanthus cultivation by 25.5–45.3%, whereas CaCl2-extractible TEs decreased due to complex rhizosphere processes driving plant mineral uptake, and organic carbon inputs into the rhizosphere. In the contaminated soils, miscanthus accumulated Cd, Pb and Zn mainly in roots (BCF in roots: Cd " Zn > Pb), while strongly reducing the transfer of these elements from soil to all organs and from roots to rhizomes, stems and leaves (average TFs: 0.01–0.06, 0.11–1.15 and 0.09–0.79 corresponding to Cd, Pb and Zn respectively). Therefore, miscanthus could be considered a TE-excluder, hence a potential candidate crop for coupling phytostabilization and biomass production on the studied Metaleurop TE-contaminated soils.},
note = {ACL},
keywords = {ER4},
pubstate = {published},
tppubtype = {article}
}
Phytomanagement is proposed as a cost-effective and environmentally-friendly suggestion for sustainable use of large metal-contaminated areas. In the current work, the energy crop miscanthus (Miscanthus × giganteus) was grown in ex situ conditions on agricultural soils presenting a Cd, Pb and Zn contamination gradient. After 93 days of culture, shoot and root growth parameters were measured. Soils and plants were sampled as well to study the TE accumulation in miscanthus and the effects of this plant on TE mobility in soils. Results demonstrated that miscanthus growth depended more on the soils silt content rather than TE-contamination level. Moreover, soil organic carbon at T93 increased in the soils after miscanthus cultivation by 25.5–45.3%, whereas CaCl2-extractible TEs decreased due to complex rhizosphere processes driving plant mineral uptake, and organic carbon inputs into the rhizosphere. In the contaminated soils, miscanthus accumulated Cd, Pb and Zn mainly in roots (BCF in roots: Cd " Zn > Pb), while strongly reducing the transfer of these elements from soil to all organs and from roots to rhizomes, stems and leaves (average TFs: 0.01–0.06, 0.11–1.15 and 0.09–0.79 corresponding to Cd, Pb and Zn respectively). Therefore, miscanthus could be considered a TE-excluder, hence a potential candidate crop for coupling phytostabilization and biomass production on the studied Metaleurop TE-contaminated soils. |
2021Journal Article ER4 Auteurs : Perouel, Guillaume; Keirsbulck, Marion; Chaigneau, Thomas; Delannoy, Matthieu; Esteve, Williams; Bot, Barbara Le; Noack, Yves; Pelfrêne, Aurélie; Glorennec, Philippe Évaluation de l’exposition et valeurs de référence pour les poussières sédimentées dans les environnements intérieurs In: Environnement, Risques & Santé, vol. 20, no. 4, pp. 383–388, 2021, ISSN: 1635-0421, (ACL). Abstract | Links @article{guillaume_perouel_evaluation_2021,
title = {Évaluation de l’exposition et valeurs de référence pour les poussières sédimentées dans les environnements intérieurs},
author = {Guillaume Perouel and Marion Keirsbulck and Thomas Chaigneau and Matthieu Delannoy and Williams Esteve and Barbara Le Bot and Yves Noack and Aurélie Pelfrêne and Philippe Glorennec},
doi = {10.1684/ers.2021.1569},
issn = {1635-0421},
year = {2021},
date = {2021-07-01},
urldate = {2021-07-01},
journal = {Environnement, Risques & Santé},
volume = {20},
number = {4},
pages = {383--388},
abstract = {textlessptextgreaterLes évaluations des risques sanitaires des substances chimiques considèrent de plus en plus fréquemment les expositions agrégées et/ou cumulées afin de caractériser de manière la plus réaliste les risques sanitaires pour la population.textless/ptextgreatertextlessptextgreaterL’exposition environnementale aux substances chimiques textitvia la poussière sédimentée sur les surfaces intérieures doit-elle être prise en compte et de quelle manière ?textless/ptextgreatertextlessptextgreaterLa population est exposée aux substances chimiques présentes dans la poussière sédimentée par ingestion, inhalation et contact cutané. L’ingestion semble la voie d’exposition la plus importante, et la seule à pouvoir être estimée au vu des connaissances actuelles. Pour la mesure, il est recommandé d’utiliser la technique de prélèvement par aspiration sur une surface déterminée, suivie d’un tamisage à 250 μm (taille maximum des particules adhérant aux mains) afin de documenter les concentrations massique et surfacique. La mesure de la bioaccessibilité orale permettrait de mieux estimer l’exposition mais les méthodes ne sont pas validées à ce jour pour la majorité des composés. Les valeurs guides pour les poussières intérieures (VGPI) sont pertinentes si l’exposition textitvia la poussière est non négligeable pour une fraction de la population. Elles pourraient être élaborées simplement en allouant à la poussière une fraction de la valeur toxicologique de référence.textless/ptextgreater},
note = {ACL},
keywords = {ER4},
pubstate = {published},
tppubtype = {article}
}
textlessptextgreaterLes évaluations des risques sanitaires des substances chimiques considèrent de plus en plus fréquemment les expositions agrégées et/ou cumulées afin de caractériser de manière la plus réaliste les risques sanitaires pour la population.textless/ptextgreatertextlessptextgreaterL’exposition environnementale aux substances chimiques textitvia la poussière sédimentée sur les surfaces intérieures doit-elle être prise en compte et de quelle manière ?textless/ptextgreatertextlessptextgreaterLa population est exposée aux substances chimiques présentes dans la poussière sédimentée par ingestion, inhalation et contact cutané. L’ingestion semble la voie d’exposition la plus importante, et la seule à pouvoir être estimée au vu des connaissances actuelles. Pour la mesure, il est recommandé d’utiliser la technique de prélèvement par aspiration sur une surface déterminée, suivie d’un tamisage à 250 μm (taille maximum des particules adhérant aux mains) afin de documenter les concentrations massique et surfacique. La mesure de la bioaccessibilité orale permettrait de mieux estimer l’exposition mais les méthodes ne sont pas validées à ce jour pour la majorité des composés. Les valeurs guides pour les poussières intérieures (VGPI) sont pertinentes si l’exposition textitvia la poussière est non négligeable pour une fraction de la population. Elles pourraient être élaborées simplement en allouant à la poussière une fraction de la valeur toxicologique de référence.textless/ptextgreater |
2021Journal Article ER4 Auteurs : Pelfrêne, Aurélie; Douay, Francis La pollution des sols des potagers et la production de fruits et de légumes In: Jardins de France, no. 662, 2021, (ACLN). Links @article{PelfreneDouay2021,
title = {La pollution des sols des potagers et la production de fruits et de légumes},
author = {Aurélie Pelfrêne and Francis Douay},
url = {https://www.jardinsdefrance.org/la-pollution-des-sols-des-potagers-et-la-production-de-fruits-et-de-legumes/},
year = {2021},
date = {2021-01-01},
journal = {Jardins de France},
number = {662},
note = {ACLN},
keywords = {ER4},
pubstate = {published},
tppubtype = {article}
}
|
2021Journal Article ER4 Auteurs : Glorennec, Philippe; Shendell, Derek G.; Rasmussen, Pat E.; Waeber, Roger; Egeghy, Peter; Azuma, Kenichi; Pelfrêne, Aurélie; Bot, Barbara Le; Esteve, Williams; Perouel, Guillaume; Pernelet-Joly, Valérie; Noack, Y.; Delannoy, Mathieu; Keirsbulck, Marion; Mandin, Corinne Toward setting public health guidelines for chemicals in indoor settled dust? In: Indoor Air, vol. 31, no. 1, pp. 112-115, 2021, (ACL). Links @article{glorennec:hal-02926293,
title = {Toward setting public health guidelines for chemicals in indoor settled dust?},
author = {Philippe Glorennec and Derek G. Shendell and Pat E. Rasmussen and Roger Waeber and Peter Egeghy and Kenichi Azuma and Aurélie Pelfrêne and Barbara Le Bot and Williams Esteve and Guillaume Perouel and Valérie Pernelet-Joly and Y. Noack and Mathieu Delannoy and Marion Keirsbulck and Corinne Mandin},
url = {https://hal.archives-ouvertes.fr/hal-02926293},
doi = {10.1111/ina.12722},
year = {2021},
date = {2021-01-01},
urldate = {2021-01-01},
journal = {Indoor Air},
volume = {31},
number = {1},
pages = {112-115},
publisher = {Wiley},
note = {ACL},
keywords = {ER4},
pubstate = {published},
tppubtype = {article}
}
|
2021Conference ER4 Auteurs : Pelfrêne, Aurélie Simplified method for oral bioaccessibility of metal(loid)s in soils SOILveR coffee break meeting, Soil and land research funding platform for Europe, Online, 2021, (COM). @conference{Pelfrene2021,
title = {Simplified method for oral bioaccessibility of metal(loid)s in soils},
author = {Aurélie Pelfrêne},
year = {2021},
date = {2021-05-31},
urldate = {2021-05-31},
booktitle = {SOILveR coffee break meeting, Soil and land research funding platform for Europe},
address = {Online},
note = {COM},
keywords = {ER4},
pubstate = {published},
tppubtype = {conference}
}
|
2020Journal Article ER4 Auteurs : Louzon, Maxime; Pelfrêne, Aurélie; Pauget, Benjamin; Gimbert, Frédéric; Crini, Nadia; Douay, Francis; De-Vaufleury, Annette Bioaccessibility of metal(loid)s in soils to humans and their bioavailability to snails: a way to associate human health and ecotoxicological risk assessment? In: Journal of Hazardous Materials, vol. 384, pp. 121432, 2020, (ACL). Abstract @article{Louzon2020,
title = {Bioaccessibility of metal(loid)s in soils to humans and their bioavailability to snails: a way to associate human health and ecotoxicological risk assessment?},
author = {Maxime Louzon and Aurélie Pelfrêne and Benjamin Pauget and Frédéric Gimbert and Nadia Crini and Francis Douay and Annette De-Vaufleury},
year = {2020},
date = {2020-01-01},
journal = {Journal of Hazardous Materials},
volume = {384},
pages = {121432},
abstract = {Human health risk assessment (HHRA) and ecotoxicological risk assessment
(ERA) of contaminated soils are frequently performed separately and
based on total soil concentrations without considering the concepts
of mobility, bioaccessibility and bioavailability. However, some
chemical and biological assays rarely used in combination can be
applied to more accurately assess the exposure of organisms to metal(loid)s
and thus to better estimate the links between soil contamination
and effects. For humans, the unified bioaccessibility method (UBM)
assesses oral bioaccessibility, while for soil fauna such as land
snails, the bioaccumulation test reflects the bioavailability of
contaminants. The aim of this study is to explore the relationship
between oral bioaccessibility and the bioavailability of arsenic,
cadmium and lead in twenty-nine contaminated soils. The results show
a modulation of bioaccumulation and bioaccessibility of metal(loid)s
by soil physicochemical parameters (organic matter especially). For
the three metal(loid)s studied, strong relationships were modelled
between the UBM and snail tests (0.77 < r²adj.<0.95), depending on
the parameters of the linear regressions (contaminant and phases
of the UBM test). The original models proposed demonstrate the feasibility
of linking bioaccessibility to humans and bioavailability to snails
and the relevance of their association for an integrative risk assessment
of contaminated soils.},
note = {ACL},
keywords = {ER4},
pubstate = {published},
tppubtype = {article}
}
Human health risk assessment (HHRA) and ecotoxicological risk assessment
(ERA) of contaminated soils are frequently performed separately and
based on total soil concentrations without considering the concepts
of mobility, bioaccessibility and bioavailability. However, some
chemical and biological assays rarely used in combination can be
applied to more accurately assess the exposure of organisms to metal(loid)s
and thus to better estimate the links between soil contamination
and effects. For humans, the unified bioaccessibility method (UBM)
assesses oral bioaccessibility, while for soil fauna such as land
snails, the bioaccumulation test reflects the bioavailability of
contaminants. The aim of this study is to explore the relationship
between oral bioaccessibility and the bioavailability of arsenic,
cadmium and lead in twenty-nine contaminated soils. The results show
a modulation of bioaccumulation and bioaccessibility of metal(loid)s
by soil physicochemical parameters (organic matter especially). For
the three metal(loid)s studied, strong relationships were modelled
between the UBM and snail tests (0.77 < r²adj.<0.95), depending on
the parameters of the linear regressions (contaminant and phases
of the UBM test). The original models proposed demonstrate the feasibility
of linking bioaccessibility to humans and bioavailability to snails
and the relevance of their association for an integrative risk assessment
of contaminated soils. |
2020Journal Article ER4 Auteurs : Janus, Adeline; Waterlot, Christophe; Douay, Francis; Pelfrêne, Aurélie Ex situ evaluation of the effects of biochars on environmental and toxicological availabilities of metals and polycyclic aromatic hydrocarbons In: Environmental Science and Pollution Research, vol. 27, pp. 1852–1869, 2020, (ACL). Abstract @article{Janus2020,
title = {Ex situ evaluation of the effects of biochars on environmental and toxicological availabilities of metals and polycyclic aromatic hydrocarbons},
author = {Adeline Janus and Christophe Waterlot and Francis Douay and Aurélie Pelfrêne},
year = {2020},
date = {2020-01-01},
journal = {Environmental Science and Pollution Research},
volume = {27},
pages = {1852–1869},
abstract = {The present study experimented five biochars, one made from wood (400
°C, 12 h) and four made from miscanthus cultivated on contaminated
soils (temperature 400/600 °C, duration 45/90 min). They were used
as amendments at a 2% application rate on soil, cultivated or not
cultivated with ryegrass, contaminated with (i) metals (Cd, Pb, and
Zn), (ii) eight polycyclic aromatic hydrocarbons (PAHs), and (iii)
a mix of metals and PAHs. The objectives were (i) to compare the
effectiveness of the five biochars on soil parameters and pollutant
availability and (ii) to determine the influence of soil multicontamination
and ryegrass cultivation on biochar effectiveness. The results showed
that biochar application did not necessarily lead to lower pollutant
extractability and metal bioaccessibility. However, differences were
highlighted between the biochars. The miscanthus biochars produced
at 600 °C (BM600) showed higher effectiveness at decreasing metal
extractability than the miscanthus biochars produced at 400 °C (BM400)
due to its better sorption characteristics. In addition, ryegrass
cultivation did not impact pollutant availability but modified metal
bioaccessibility, especially for the soil amended with the BM600
and the woody biochar. Moreover, the presence of PAHs also negatively
impacted the metal bioaccessibility in the soil amended with the
BM600, and, on the contrary, positively impacted it in the soil amended
with the BM400. Complementary studies are therefore necessary to
understand the mechanisms involved, particularly in a context where
soils requiring remediation operations are often multicontaminated
and vegetated.},
note = {ACL},
keywords = {ER4},
pubstate = {published},
tppubtype = {article}
}
The present study experimented five biochars, one made from wood (400
°C, 12 h) and four made from miscanthus cultivated on contaminated
soils (temperature 400/600 °C, duration 45/90 min). They were used
as amendments at a 2% application rate on soil, cultivated or not
cultivated with ryegrass, contaminated with (i) metals (Cd, Pb, and
Zn), (ii) eight polycyclic aromatic hydrocarbons (PAHs), and (iii)
a mix of metals and PAHs. The objectives were (i) to compare the
effectiveness of the five biochars on soil parameters and pollutant
availability and (ii) to determine the influence of soil multicontamination
and ryegrass cultivation on biochar effectiveness. The results showed
that biochar application did not necessarily lead to lower pollutant
extractability and metal bioaccessibility. However, differences were
highlighted between the biochars. The miscanthus biochars produced
at 600 °C (BM600) showed higher effectiveness at decreasing metal
extractability than the miscanthus biochars produced at 400 °C (BM400)
due to its better sorption characteristics. In addition, ryegrass
cultivation did not impact pollutant availability but modified metal
bioaccessibility, especially for the soil amended with the BM600
and the woody biochar. Moreover, the presence of PAHs also negatively
impacted the metal bioaccessibility in the soil amended with the
BM600, and, on the contrary, positively impacted it in the soil amended
with the BM400. Complementary studies are therefore necessary to
understand the mechanisms involved, particularly in a context where
soils requiring remediation operations are often multicontaminated
and vegetated. |
2020Journal Article ER4 Auteurs : Nguyen, Van-Xuan; Douay, Francis; Mamindy-Pajany, Yannick; Alary, Claire; Pelfrêne, Aurelie Environmental availability and oral bioaccessibility of Cd and Pb in anthroposols from dredged river sediments In: Environmental Science and Pollution Research, vol. 27, no. 1, pp. 622-635, 2020, (ACL). Abstract @article{Nguyen2020,
title = {Environmental availability and oral bioaccessibility of Cd and Pb in anthroposols from dredged river sediments},
author = {Van-Xuan Nguyen and Francis Douay and Yannick Mamindy-Pajany and Claire Alary and Aurelie Pelfrêne},
year = {2020},
date = {2020-01-01},
journal = {Environmental Science and Pollution Research},
volume = {27},
number = {1},
pages = {622-635},
abstract = {Dredging and disposal of sediments onto land sites is a common practice
in urban and industrial areas that can present environmental and
health risks when the sediments contain metallic elements. The aim
of this study was to characterise and study the environmental and
toxicological availability of Cd and Pb in anthroposols from dredged
river sediments. To do this, 67 surface samples spread over 12 sediment
disposal sites in northern France were studied. The results showed
substantial heterogeneity for this matrix in terms of physicochemical
parameters and contamination degree; however, ascending hierarchical
clustering made it possible to classify the samples into eight groups.
For each group, the mobile fraction of Cd and Pb was studied using
single EDTA extraction, solid-phase distribution was analysed with
sequential extractions and toxicological availability was assessed
with the oral bioaccessibility test. The results showed that (i)
Cd had a higher environmental and toxicological availability than
Pb; (ii) this availability depends on the physicochemical characteristics
of the matrix; and (iii) it is necessary to take into account the
environmental and toxicological availability of contaminants when
requalifying these sites in order to propose appropriate management
measures. In the first years after sediment disposal, it would appear
that the environmental and toxicological availability of Cd and Pb
increased (from 52.5 to 71.8% and from 28.9 to 48.9%, respectively,
by using EDTA and from 50.2 to 68.5% for Cd with the bioaccessibility
test). Further studies would therefore be required to confirm this
trend and understand the mechanisms involved.},
note = {ACL},
keywords = {ER4},
pubstate = {published},
tppubtype = {article}
}
Dredging and disposal of sediments onto land sites is a common practice
in urban and industrial areas that can present environmental and
health risks when the sediments contain metallic elements. The aim
of this study was to characterise and study the environmental and
toxicological availability of Cd and Pb in anthroposols from dredged
river sediments. To do this, 67 surface samples spread over 12 sediment
disposal sites in northern France were studied. The results showed
substantial heterogeneity for this matrix in terms of physicochemical
parameters and contamination degree; however, ascending hierarchical
clustering made it possible to classify the samples into eight groups.
For each group, the mobile fraction of Cd and Pb was studied using
single EDTA extraction, solid-phase distribution was analysed with
sequential extractions and toxicological availability was assessed
with the oral bioaccessibility test. The results showed that (i)
Cd had a higher environmental and toxicological availability than
Pb; (ii) this availability depends on the physicochemical characteristics
of the matrix; and (iii) it is necessary to take into account the
environmental and toxicological availability of contaminants when
requalifying these sites in order to propose appropriate management
measures. In the first years after sediment disposal, it would appear
that the environmental and toxicological availability of Cd and Pb
increased (from 52.5 to 71.8% and from 28.9 to 48.9%, respectively,
by using EDTA and from 50.2 to 68.5% for Cd with the bioaccessibility
test). Further studies would therefore be required to confirm this
trend and understand the mechanisms involved. |
2020Journal Article ER4 Auteurs : Bidar, Géraldine; Pelfrêne, Aurélie; Schwartz, Christophe; Waterlot, Christophe; Sahmer, Karin; Marot, Franck; Douay, Francis Urban kitchen gardens: Effect of the soil contamination and parameters on the trace element accumulation in vegetables – A review In: Science of the Total Environment, vol. 738, pp. 139569, 2020, (ACL). Abstract @article{Bidar2020,
title = {Urban kitchen gardens: Effect of the soil contamination and parameters on the trace element accumulation in vegetables – A review},
author = {Géraldine Bidar and Aurélie Pelfrêne and Christophe Schwartz and Christophe Waterlot and Karin Sahmer and Franck Marot and Francis Douay},
year = {2020},
date = {2020-01-01},
journal = {Science of the Total Environment},
volume = {738},
pages = {139569},
abstract = {Trace element contaminants in kitchen garden soils can contribute
to human exposure through the consumption of homegrown vegetables.
In urban areas, these soils can be contaminated to various degrees
by trace element (TE). They are characterized by a great variability
in their physicochemical parameters due to the high anthropization
level, the wide variety and combination of disturbance sources, aswell
as the diversity of cultivation practices and the large range of
contamination levels. Pollutants can be taken up by vegetables cultivated
in these soils and be concentrated in their edible parts. In this
review, the behavior of vegetables cultivated in contaminated kitchen
gardens is assessed through six examples of the most widely cultivated
vegetables (lettuce, tomato, bean, carrot, radish, potato). The role
of soil parameters that could influence the uptake of As, Cd, Cr,
Ni, Pb, and Zn by these vegetables is also discussed.},
note = {ACL},
keywords = {ER4},
pubstate = {published},
tppubtype = {article}
}
Trace element contaminants in kitchen garden soils can contribute
to human exposure through the consumption of homegrown vegetables.
In urban areas, these soils can be contaminated to various degrees
by trace element (TE). They are characterized by a great variability
in their physicochemical parameters due to the high anthropization
level, the wide variety and combination of disturbance sources, aswell
as the diversity of cultivation practices and the large range of
contamination levels. Pollutants can be taken up by vegetables cultivated
in these soils and be concentrated in their edible parts. In this
review, the behavior of vegetables cultivated in contaminated kitchen
gardens is assessed through six examples of the most widely cultivated
vegetables (lettuce, tomato, bean, carrot, radish, potato). The role
of soil parameters that could influence the uptake of As, Cd, Cr,
Ni, Pb, and Zn by these vegetables is also discussed. |
2020Journal Article ER4 Auteurs : Pelfrêne, Aurélie; Sahmer, Karin; Waterlot, Christophe; Glorennec, Philippe; Douay, Francis; Le-Bot, Barbara Evaluation of single-extraction methods to estimate the oral bioaccessibility of metal(loid)s in soils In: Science of the Total Environment, vol. 727, pp. 138553, 2020, (ACL). Abstract @article{Pelfrene2020,
title = {Evaluation of single-extraction methods to estimate the oral bioaccessibility of metal(loid)s in soils},
author = {Aurélie Pelfrêne and Karin Sahmer and Christophe Waterlot and Philippe Glorennec and Francis Douay and Barbara Le-Bot},
year = {2020},
date = {2020-01-01},
journal = {Science of the Total Environment},
volume = {727},
pages = {138553},
abstract = {Incidental ingestion of polluted soil particles exposes the population
to toxic metal(loid)s. To refine the methods of exposure and risk
assessment, it is relevant to use bioaccessible concentrations of
metal(loid)s determined via in vitro digestion methods. However,
some validated methods are complex and costly, involving high technical
skills and numerous reagents. The objective of the present study
was to evaluate the suitability of four simple chemical extractions
to mimic the bioaccessible fraction of As, Cd, and Pb in the gastric
(G) and gastrointestinal (GI) phases obtained using the validated
UBM (unified bioaccessibility method) test. Acetic acid (0.11 M),
citric acid (0.11M), EDTA (0.16 M), and hydrochloric acid (HCl, 0.65%)were
separately tested in 201 soil sampleswith a wide range of physicochemical
parameters and metal(loid)s concentrations. Significant linear relationships
were observed with HCl, EDTA, and to a lesser extent with citric
acid. For the cheaper HCl method, correlations with the UBM ranged
from 0.91 to 0.99 for the G phase and from 0.72 to 0.97 for the GI
phase. This test can be used at least as a first-tier screening to
assess the oral bioaccessibility of As, Cd, and Pb.},
note = {ACL},
keywords = {ER4},
pubstate = {published},
tppubtype = {article}
}
Incidental ingestion of polluted soil particles exposes the population
to toxic metal(loid)s. To refine the methods of exposure and risk
assessment, it is relevant to use bioaccessible concentrations of
metal(loid)s determined via in vitro digestion methods. However,
some validated methods are complex and costly, involving high technical
skills and numerous reagents. The objective of the present study
was to evaluate the suitability of four simple chemical extractions
to mimic the bioaccessible fraction of As, Cd, and Pb in the gastric
(G) and gastrointestinal (GI) phases obtained using the validated
UBM (unified bioaccessibility method) test. Acetic acid (0.11 M),
citric acid (0.11M), EDTA (0.16 M), and hydrochloric acid (HCl, 0.65%)were
separately tested in 201 soil sampleswith a wide range of physicochemical
parameters and metal(loid)s concentrations. Significant linear relationships
were observed with HCl, EDTA, and to a lesser extent with citric
acid. For the cheaper HCl method, correlations with the UBM ranged
from 0.91 to 0.99 for the G phase and from 0.72 to 0.97 for the GI
phase. This test can be used at least as a first-tier screening to
assess the oral bioaccessibility of As, Cd, and Pb. |
2020Conference ER4 Auteurs : Pauget, Benjamin; Louzon, Maxime; Gimbert, Frédéric; Pelfrêne, Aurélie; De-Vaufleury, Annette La bioaccessibilité et la biodisponibilité, deux outils pour une évaluation des risques intégrative (projet COMBINE) Journée Technique sur les Risques environnementaux et reconversion des friches, Lyon, France, 6 novembre 2020, 2020, (COM). @conference{Pauget2020,
title = {La bioaccessibilité et la biodisponibilité, deux outils pour une évaluation des risques intégrative (projet COMBINE)},
author = {Benjamin Pauget and Maxime Louzon and Frédéric Gimbert and Aurélie Pelfrêne and Annette De-Vaufleury},
year = {2020},
date = {2020-01-01},
booktitle = {Journée Technique sur les Risques environnementaux et reconversion des friches, Lyon, France, 6 novembre 2020},
note = {COM},
keywords = {ER4},
pubstate = {published},
tppubtype = {conference}
}
|
2020Conference ER4 Auteurs : Pelfrêne, Aurélie Une méthode simplifiée pour estimer la bioaccessibilité orale des polluants métalliques dans les sols Journée Technique sur les Risques environnementaux et reconversion des friches, Lyon, France, 6 novembre 2020, 2020, (COM). @conference{Pelfrene2020a,
title = {Une méthode simplifiée pour estimer la bioaccessibilité orale des polluants métalliques dans les sols},
author = {Aurélie Pelfrêne},
year = {2020},
date = {2020-01-01},
booktitle = {Journée Technique sur les Risques environnementaux et reconversion des friches, Lyon, France, 6 novembre 2020},
note = {COM},
keywords = {ER4},
pubstate = {published},
tppubtype = {conference}
}
|
2020Book ER4 Auteurs : Pelfrêne, Aurelie; Bidar, Géraldine; Détriché, Sébastien; Waterlot, Christophe; Pruvot, Christelle; Douay, Francis Spécificités des potagers en contexte (péri)urbain au lourd passé industriel 2020, (OS). @book{Pelfrene2020c,
title = {Spécificités des potagers en contexte (péri)urbain au lourd passé industriel},
author = {Aurelie Pelfrêne and Géraldine Bidar and Sébastien Détriché and Christophe Waterlot and Christelle Pruvot and Francis Douay},
year = {2020},
date = {2020-01-01},
booktitle = {in "Les sols urbains sont-ils cultivables ?" (Editions Quae, Collection Matière à débattres & décider)},
note = {OS},
keywords = {ER4},
pubstate = {published},
tppubtype = {book}
}
|
2020Conference ER4 Auteurs : Louzon, Maxime; Pauget, Benjamin; Pelfrêne, Aurélie; Crini, Nadia; Gimbert, Frédéric; Douay, Francis; Amiot, Caroline; Rieffel, Dominique; De-Vaufleury, Annette COMBINE – Coupler des indicateurs chimiques et biologiques pour une évaluation intégrative des risques sanitaires et environnementaux Journée Technique sur les Risques environnementaux et reconversion des friches, Lyon, France, 6 novembre 2020, 2020, (COM). @conference{Louzon2020b,
title = {COMBINE – Coupler des indicateurs chimiques et biologiques pour une évaluation intégrative des risques sanitaires et environnementaux},
author = {Maxime Louzon and Benjamin Pauget and Aurélie Pelfrêne and Nadia Crini and Frédéric Gimbert and Francis Douay and Caroline Amiot and Dominique Rieffel and Annette De-Vaufleury},
year = {2020},
date = {2020-01-01},
urldate = {2020-01-01},
booktitle = {Journée Technique sur les Risques environnementaux et reconversion des friches, Lyon, France, 6 novembre 2020},
note = {COM},
keywords = {ER4},
pubstate = {published},
tppubtype = {conference}
}
|
2019Journal Article ER4 Auteurs : Bidar, Géraldine; Pelfrêne, Aurélie; Louvel, Brice; Janus, Adeline; Douay, Francis Influence of amendments on metal environmental and toxicological availability in highly contaminated brownfield and agricultural soils In: Environmental Science and Pollution Research, vol. 26, pp. 33086–33108, 2019, (ACL). Abstract @article{Bidar2019,
title = {Influence of amendments on metal environmental and toxicological availability in highly contaminated brownfield and agricultural soils},
author = {Géraldine Bidar and Aurélie Pelfrêne and Brice Louvel and Adeline Janus and Francis Douay},
year = {2019},
date = {2019-01-01},
journal = {Environmental Science and Pollution Research},
volume = {26},
pages = {33086–33108},
abstract = {The immobilizing effects of wood biochar (BW2%) and iron grit (Z1%)
applied alone or in combination (BW2% + Z1%) to agricultural (M750)
and brownfield (MAZ) soils highly contaminated by metals were assessed
in a greenhouse experiment. The results showed that Z1% and BW2%
+ Z1% were the most efficient amendments to reduce Cd, Cu, Pb, and
Zn mobility, environmental availability, and phytoavailability in
the M750 soil. The oxidation of Z1% allowed part of the Cu and Zn
pools present in exchangeable or carbonate-bound forms (labile fraction)
to complex in less mobile forms. In this soil, the metal chemical
extractions (0.01 M CaCl2 and 0.05 M EDTA) and the DGT (diffusive
gradient in thin films) devices to assess metal in soil solution
and soil pore water (SPW) also highlighted the immobilizing characteristic
of Z1%. In most cases, the addition of BW2% to Z1% (BW2% + Z1%) did
not improve this effect, except for the dissolved Pb and Zn concentrations
in the M750 soil solution. It was also observed that Cd, Pb, and
Zn passed throughout DGT mimicking the biological cell membrane were
reduced by all amendments of the M750 soil corroborating metal concentrations
measured in rye grass shoots. In the MAZ soil, metals were less available
as shown by their low extractability rate, low capacity of metal
resupply from the solid phase to pore water, and low phytoavailability.
The poor metal availability could be explained by the high levels
of carbonate and organic matter contents in this soil. Nevertheless,
a decrease of the Cu environmental availability and the Cu concentrations
in rye grass shoots grown on the MAZ soil was also observed in the
soil amended with Z1% alone or in combination with BW2%. From a health
point of view, the most effective amendment to reduce human exposure
through ingestion of soil particles for the M750 and MAZ soils was
BW2% for Cd and BW2% + Z1% for Pb. However, the presence of rye grass
minimized the amendments’ beneficial effects.},
note = {ACL},
keywords = {ER4},
pubstate = {published},
tppubtype = {article}
}
The immobilizing effects of wood biochar (BW2%) and iron grit (Z1%)
applied alone or in combination (BW2% + Z1%) to agricultural (M750)
and brownfield (MAZ) soils highly contaminated by metals were assessed
in a greenhouse experiment. The results showed that Z1% and BW2%
+ Z1% were the most efficient amendments to reduce Cd, Cu, Pb, and
Zn mobility, environmental availability, and phytoavailability in
the M750 soil. The oxidation of Z1% allowed part of the Cu and Zn
pools present in exchangeable or carbonate-bound forms (labile fraction)
to complex in less mobile forms. In this soil, the metal chemical
extractions (0.01 M CaCl2 and 0.05 M EDTA) and the DGT (diffusive
gradient in thin films) devices to assess metal in soil solution
and soil pore water (SPW) also highlighted the immobilizing characteristic
of Z1%. In most cases, the addition of BW2% to Z1% (BW2% + Z1%) did
not improve this effect, except for the dissolved Pb and Zn concentrations
in the M750 soil solution. It was also observed that Cd, Pb, and
Zn passed throughout DGT mimicking the biological cell membrane were
reduced by all amendments of the M750 soil corroborating metal concentrations
measured in rye grass shoots. In the MAZ soil, metals were less available
as shown by their low extractability rate, low capacity of metal
resupply from the solid phase to pore water, and low phytoavailability.
The poor metal availability could be explained by the high levels
of carbonate and organic matter contents in this soil. Nevertheless,
a decrease of the Cu environmental availability and the Cu concentrations
in rye grass shoots grown on the MAZ soil was also observed in the
soil amended with Z1% alone or in combination with BW2%. From a health
point of view, the most effective amendment to reduce human exposure
through ingestion of soil particles for the M750 and MAZ soils was
BW2% for Cd and BW2% + Z1% for Pb. However, the presence of rye grass
minimized the amendments’ beneficial effects. |
2019Journal Article ER4 Auteurs : Dumat, Camille; Pelfrêne, Aurélie; Shahid, Muhammad Environment-health link in a context of urban agricultures: studies of oral exposure to pollutants in order promote the human health In: Environmental Science and Pollution Research, vol. 26, no. 20, pp. 20015-20017, 2019, (ACL). Abstract @article{Dumat2019,
title = {Environment-health link in a context of urban agricultures: studies of oral exposure to pollutants in order promote the human health},
author = {Camille Dumat and Aurélie Pelfrêne and Muhammad Shahid},
year = {2019},
date = {2019-01-01},
journal = {Environmental Science and Pollution Research},
volume = {26},
number = {20},
pages = {20015-20017},
abstract = {This ESPR special issue includes a selection of papers presented at
the international congress “Sustainable Urban Agriculture: Vector
for the Ecological Transition” (UA&ET), which is focused in a special
session on the link between environment and human health, and which
was held on June 2017 in Toulouse, France.},
note = {ACL},
keywords = {ER4},
pubstate = {published},
tppubtype = {article}
}
This ESPR special issue includes a selection of papers presented at
the international congress “Sustainable Urban Agriculture: Vector
for the Ecological Transition” (UA&ET), which is focused in a special
session on the link between environment and human health, and which
was held on June 2017 in Toulouse, France. |
2019Conference ER4 Auteurs : Le-Bot, Barbara; Glorennec, Philippe; Waterlot, Christophe; Douay, Francis; Pelfrêne, Aurélie Simplified method for oral bioaccessibility of metal(loid)s in soils and alternative to the Unified Barge Method International Societies of Exposure Science (ISES) and Indoor Air Quality and Climate (ISIAQ), 18-22 August 2019, Kaunas (Lithuania), 2019, (AFF). @conference{Le-Bot2019,
title = {Simplified method for oral bioaccessibility of metal(loid)s in soils and alternative to the Unified Barge Method},
author = {Barbara Le-Bot and Philippe Glorennec and Christophe Waterlot and Francis Douay and Aurélie Pelfrêne},
year = {2019},
date = {2019-01-01},
booktitle = {International Societies of Exposure Science (ISES) and Indoor Air Quality and Climate (ISIAQ), 18-22 August 2019, Kaunas (Lithuania)},
note = {AFF},
keywords = {ER4},
pubstate = {published},
tppubtype = {conference}
}
|
2019Conference ER4 Auteurs : Louzon, Maxime; Pelfrêne, Aurélie; Pauget, Benjamin; Gimbert, Frédéric; Crini, Nadia; Rieffel, Dominique; Amiot, Caroline; Douay, Francis; De-Vaufleury, Annette Assessment of metal(loid) bioavailability for landsnails and human bioaccessibility: a new pathway to build bridges between ecotoxicological and human health risk assessment of contaminated soils SETAC Europe, 29th Annual meeting, 26-30 May 2019, Helsinki (Finland), 2019, (ACTI). @conference{Louzon2019,
title = {Assessment of metal(loid) bioavailability for landsnails and human bioaccessibility: a new pathway to build bridges between ecotoxicological and human health risk assessment of contaminated soils},
author = {Maxime Louzon and Aurélie Pelfrêne and Benjamin Pauget and Frédéric Gimbert and Nadia Crini and Dominique Rieffel and Caroline Amiot and Francis Douay and Annette De-Vaufleury},
year = {2019},
date = {2019-01-01},
booktitle = {SETAC Europe, 29th Annual meeting, 26-30 May 2019, Helsinki (Finland)},
note = {ACTI},
keywords = {ER4},
pubstate = {published},
tppubtype = {conference}
}
|
2019Conference ER4 Auteurs : Louzon, Maxime; Pauget, Barbara; Gimbert, Frédéric; Pelfrêne, Aurélie; De-Vaufleury, Annette COMBINE – Coupler des indicateurs chimiques et biologiques pour une évaluation intégrative des risques sanitaires et environnementaux Journée technique « Prise en compte des fonctions écosystémiques du sol et du sous-sol en contexte de réaménagement urbain », 14 mai 2019, Lyon, 2019, (ACTN). @conference{Louzon2019a,
title = {COMBINE – Coupler des indicateurs chimiques et biologiques pour une évaluation intégrative des risques sanitaires et environnementaux},
author = {Maxime Louzon and Barbara Pauget and Frédéric Gimbert and Aurélie Pelfrêne and Annette De-Vaufleury},
year = {2019},
date = {2019-01-01},
booktitle = {Journée technique « Prise en compte des fonctions écosystémiques du sol et du sous-sol en contexte de réaménagement urbain », 14 mai 2019, Lyon},
note = {ACTN},
keywords = {ER4},
pubstate = {published},
tppubtype = {conference}
}
|
2019Conference ER4 Auteurs : Pelfrêne, Aurélie Simplified method for oral bioaccessibility of metal(loid)s in soils ISO/TC 190/SC 7/WG 4 meeting, 15 October 2019, Aveiro (Portugal), 2019, (ACTI). Abstract @conference{Pelfrene2019,
title = {Simplified method for oral bioaccessibility of metal(loid)s in soils},
author = {Aurélie Pelfrêne},
year = {2019},
date = {2019-01-01},
booktitle = {ISO/TC 190/SC 7/WG 4 meeting, 15 October 2019, Aveiro (Portugal)},
pages = {18pp},
abstract = {Objectives: Due to the complexity of in vitro methods , a simplification
of them might be a great interest for managers of Polluted Sites
and Soils Propose a first tier method as a decision making tool Evaluate
the potential suitability of chemical single extraction methods to
mimic the bioaccessible fraction of As, Cd and Pb in a wide range
of soils},
note = {ACTI},
keywords = {ER4},
pubstate = {published},
tppubtype = {conference}
}
Objectives: Due to the complexity of in vitro methods , a simplification
of them might be a great interest for managers of Polluted Sites
and Soils Propose a first tier method as a decision making tool Evaluate
the potential suitability of chemical single extraction methods to
mimic the bioaccessible fraction of As, Cd and Pb in a wide range
of soils |
2019Conference ER4 Auteurs : Pelfrêne, Aurélie; Le-Bot, Barbara; Waterlot, Christophe; Glorennec, Philippe; Sahmer, Karin; Douay, Francis Evaluation of four first tier methods to measure metal(loid) bioaccessibility in polluted soils SETAC Europe, 29th Annual meeting, 26-30 May 2019, Helsinki (Finland), 2019, (ACTI). @conference{Pelfrene2019a,
title = {Evaluation of four first tier methods to measure metal(loid) bioaccessibility in polluted soils},
author = {Aurélie Pelfrêne and Barbara Le-Bot and Christophe Waterlot and Philippe Glorennec and Karin Sahmer and Francis Douay},
year = {2019},
date = {2019-01-01},
booktitle = {SETAC Europe, 29th Annual meeting, 26-30 May 2019, Helsinki (Finland)},
note = {ACTI},
keywords = {ER4},
pubstate = {published},
tppubtype = {conference}
}
|
2019Conference ER4 Auteurs : Pelfrêne, Aurélie; Roussel, Hélène Méthode simplifiée pour la bioaccessibilité orale des métaux dans les sols Journée technique d’information et de retour d’expérience de la gestion des sites et sols pollués 7 novembre 2019, Paris, 2019, (COM). Abstract @conference{Pelfrene2019b,
title = {Méthode simplifiée pour la bioaccessibilité orale des métaux dans les sols},
author = {Aurélie Pelfrêne and Hélène Roussel},
year = {2019},
date = {2019-01-01},
booktitle = {Journée technique d’information et de retour d’expérience de la gestion des sites et sols pollués 7 novembre 2019, Paris},
abstract = {Objectifs: *En raison de la complexité des méthodes in vitro , leur
simplification pourrait présenter un fort intérêt pour les gestionnaires
SSP *Proposer une méthode en 1ère approche comme un outil d’aide
à la décision *Evaluer la pertinence de méthodes d’extractions chimiques
simples pour mimer la fraction bioaccessible fraction de As, Cd et
Pb pour une large gamme de sols},
note = {COM},
keywords = {ER4},
pubstate = {published},
tppubtype = {conference}
}
Objectifs: *En raison de la complexité des méthodes in vitro , leur
simplification pourrait présenter un fort intérêt pour les gestionnaires
SSP *Proposer une méthode en 1ère approche comme un outil d’aide
à la décision *Evaluer la pertinence de méthodes d’extractions chimiques
simples pour mimer la fraction bioaccessible fraction de As, Cd et
Pb pour une large gamme de sols |
2019Journal Article ER4 Auteurs : Pelfrêne, Aurélie; Sahmer, Karin; Grard, Olivier; Heyman, Christophe; Douay, Francis Exposition des jardiniers urbains dans un contexte industrialisé – Aspects méthodologiques In: Techniques de l’ingénieur, vol. 10 novembre 2019, no. GE1016 V1, pp. 17pp, 2019, (OV). Abstract @article{Pelfrene2019c,
title = {Exposition des jardiniers urbains dans un contexte industrialisé – Aspects méthodologiques},
author = {Aurélie Pelfrêne and Karin Sahmer and Olivier Grard and Christophe Heyman and Francis Douay},
year = {2019},
date = {2019-01-01},
journal = {Techniques de l’ingénieur},
volume = {10 novembre 2019},
number = {GE1016 V1},
pages = {17pp},
abstract = {INTRODUCTION Jusqu’à récemment le jardinage avait souvent pour vocation
principale de subvenir aux besoins alimentaires. De nos jours, les
motivations des jardiniers sont beaucoup plus variées. Outre la production
de fruits et légumes de qualité, le jardin joue aussi un rôle social
et de support de biodiversité fortement dépendant des pratiques associées
au jardinage (e.g. utilisation ou non de pesticides, intensité du
travail du sol, maintien d’habitats annexes favorables). Si le jardinage
est effectué le plus souvent en milieu rural, il se pratique de plus
en plus en milieux périurbain et urbain et peut être qualifié « d’agriculture
urbaine ». Se pose alors la question de la qualité des sols et des
productions cultivées au regard de pollutions potentielles résultant
des activités humaines actuelles et/ou passées (chauffage urbain,
circulation automobile, activités industrielles, apports de terre/remblais…).
D’une façon générale, les connaissances sur les jardins potagers
restent insuffisantes au regard de leur nombre élevé, de la diversité
de leurs contextes environnementaux, des modes de gouvernance, des
pratiques culturales et de consommation, de la complexité des réglementations
relatives à ces espaces, privatifs ou pas, et à ces productions.
L’objectif de cet article est de présenter un retour d’expérience
sur une démarche menée, en partenariat avec les services sanitaires,
dans une portion de l’ancien bassin minier du Nord-Pas-de-Calais,
région densément peuplée et avec un lourd passé industriel. La démarche,
transférable à d’autres contextes environnementaux, visait à mieux
connaître les jardins majoritairement privatifs. Elle s’étend depuis
l’étude historique du site jusqu’à la restitution auprès des jardiniers
des données acquises. Ces connaissances sont destinées à alimenter
les réflexions sur la gestion des potagers urbains en apportant des
arguments scientifiques et techniques sur les quantités produites
et consommées, les pratiques culturales des jardiniers, l’aptitude
des fruits et légumes autoproduits à accumuler des polluants métalliques.
Elles sont aussi le support de réflexions destinées à réduire l’exposition
aux polluants métalliques des jardiniers et de leur famille en lien
avec le jardinage.},
note = {OV},
keywords = {ER4},
pubstate = {published},
tppubtype = {article}
}
INTRODUCTION Jusqu’à récemment le jardinage avait souvent pour vocation
principale de subvenir aux besoins alimentaires. De nos jours, les
motivations des jardiniers sont beaucoup plus variées. Outre la production
de fruits et légumes de qualité, le jardin joue aussi un rôle social
et de support de biodiversité fortement dépendant des pratiques associées
au jardinage (e.g. utilisation ou non de pesticides, intensité du
travail du sol, maintien d’habitats annexes favorables). Si le jardinage
est effectué le plus souvent en milieu rural, il se pratique de plus
en plus en milieux périurbain et urbain et peut être qualifié « d’agriculture
urbaine ». Se pose alors la question de la qualité des sols et des
productions cultivées au regard de pollutions potentielles résultant
des activités humaines actuelles et/ou passées (chauffage urbain,
circulation automobile, activités industrielles, apports de terre/remblais…).
D’une façon générale, les connaissances sur les jardins potagers
restent insuffisantes au regard de leur nombre élevé, de la diversité
de leurs contextes environnementaux, des modes de gouvernance, des
pratiques culturales et de consommation, de la complexité des réglementations
relatives à ces espaces, privatifs ou pas, et à ces productions.
L’objectif de cet article est de présenter un retour d’expérience
sur une démarche menée, en partenariat avec les services sanitaires,
dans une portion de l’ancien bassin minier du Nord-Pas-de-Calais,
région densément peuplée et avec un lourd passé industriel. La démarche,
transférable à d’autres contextes environnementaux, visait à mieux
connaître les jardins majoritairement privatifs. Elle s’étend depuis
l’étude historique du site jusqu’à la restitution auprès des jardiniers
des données acquises. Ces connaissances sont destinées à alimenter
les réflexions sur la gestion des potagers urbains en apportant des
arguments scientifiques et techniques sur les quantités produites
et consommées, les pratiques culturales des jardiniers, l’aptitude
des fruits et légumes autoproduits à accumuler des polluants métalliques.
Elles sont aussi le support de réflexions destinées à réduire l’exposition
aux polluants métalliques des jardiniers et de leur famille en lien
avec le jardinage. |
2019Journal Article ER4 Auteurs : Pelfrêne, Aurélie; Sahmer, Karin; Waterlot, Christophe; Douay, Francis From environmental data acquisition to assessment of gardeners' exposure: feedback in an urban context highly contaminated with metals In: Environmental Science and Pollution Research, vol. 26, no. 20, pp. 20107-20120, 2019, (ACL). Abstract @article{Pelfrene2019d,
title = {From environmental data acquisition to assessment of gardeners' exposure: feedback in an urban context highly contaminated with metals},
author = {Aurélie Pelfrêne and Karin Sahmer and Christophe Waterlot and Francis Douay},
year = {2019},
date = {2019-01-01},
journal = {Environmental Science and Pollution Research},
volume = {26},
number = {20},
pages = {20107-20120},
abstract = {Although growing vegetables in urban gardens has several benefits,
some questions in relation with the safety of foods remain when the
self-production is carried out on highly contaminated garden soils.
To better assess the local population's exposure to Cd and Pb induced
by the past activities of a lead smelter, a participatory program
was initiated in 115 private kitchen gardens located in northern
France to assist gardeners in understanding their soil environment.
The challenge included contributing to the database of urban garden
soils with the collection of a large number of samples: 1525 crops
grouped into 12 types (leaf, fruiting, root, stem and bulbous vegetables,
tubers, cabbages, leguminous plants, celeriac, fresh herbs, fruits,
and berries), 708 topsoils, and 52 samples of self-produced compost.
The main results were as follows: (i) topsoils were strongly contaminated
by Cd and Pb compared to regional reference values; (ii) great variability
in physicochemical parameters and metal concentrations in topsoils;
(iii) the highest concentrations of Cd and Pb for celeriac and fresh
herbs and the lowest for fruits and fruiting vegetables; (iv) a high
percentage of vegetables that did not comply with the European foodstuff
legislation; and (v) most self-produced compost samples were strongly
contaminated. This study aimed to raise awareness and generate functional
recommendations to reduce human exposure and to provide useful data
that could be considered in other environmental contexts.},
note = {ACL},
keywords = {ER4},
pubstate = {published},
tppubtype = {article}
}
Although growing vegetables in urban gardens has several benefits,
some questions in relation with the safety of foods remain when the
self-production is carried out on highly contaminated garden soils.
To better assess the local population's exposure to Cd and Pb induced
by the past activities of a lead smelter, a participatory program
was initiated in 115 private kitchen gardens located in northern
France to assist gardeners in understanding their soil environment.
The challenge included contributing to the database of urban garden
soils with the collection of a large number of samples: 1525 crops
grouped into 12 types (leaf, fruiting, root, stem and bulbous vegetables,
tubers, cabbages, leguminous plants, celeriac, fresh herbs, fruits,
and berries), 708 topsoils, and 52 samples of self-produced compost.
The main results were as follows: (i) topsoils were strongly contaminated
by Cd and Pb compared to regional reference values; (ii) great variability
in physicochemical parameters and metal concentrations in topsoils;
(iii) the highest concentrations of Cd and Pb for celeriac and fresh
herbs and the lowest for fruits and fruiting vegetables; (iv) a high
percentage of vegetables that did not comply with the European foodstuff
legislation; and (v) most self-produced compost samples were strongly
contaminated. This study aimed to raise awareness and generate functional
recommendations to reduce human exposure and to provide useful data
that could be considered in other environmental contexts. |
2019Journal Article ER4 Auteurs : Ridoskova, Andrea; Pelfrêne, Aurélie; Douay, Francis; Pelcova, Pavlina; Smolikova, Vendula; Adam, Vojtech Bioavailability of mercury in contaminated soils assessed by the diffusive gradient in thin film technique in relation to uptake by Miscanthus x giganteus In: Environmental Toxicology and Chemistry, vol. 38, no. 2, pp. 321-328, 2019, (ACL). Abstract @article{Ridoskova2019,
title = {Bioavailability of mercury in contaminated soils assessed by the diffusive gradient in thin film technique in relation to uptake by Miscanthus x giganteus},
author = {Andrea Ridoskova and Aurélie Pelfrêne and Francis Douay and Pavlina Pelcova and Vendula Smolikova and Vojtech Adam},
year = {2019},
date = {2019-01-01},
journal = {Environmental Toxicology and Chemistry},
volume = {38},
number = {2},
pages = {321-328},
abstract = {We assessed the relationship between the diffusive gradient in thin
film (DGT) technique using the new ion-exchange resin Ambersep GT74
and the uptake of mercury (Hg) by a model plant cultivated on metal-contaminated
agricultural soils under greenhouse conditions. Based on the total
Hg content, 0.37 to 1.17% of the Hg passed to the soil porewater
from the solid phase, and 2.18 to 9.18% of the Hg is DGT-available.
These results were confirmed by calculating the R value (the ratio
of the concentrations of bioavailable Hg measured by DGT and soil
solution), which illustrated the strong bonding of Hg to the solid
phase of soil and its extremely low mobility. Only inorganic Hg(2+)
species were found in the metal-contaminated agricultural soils,
as determined by a high-performance liquid chromatography-cold vapor
atomic fluorescence spectrometry speciation analysis. The Hg was
distributed in Miscanthus x giganteus organs in the following order
for all sampling sites: roots (55-82%) >> leaves (8-27%) > stems
(7-16%) > rhizomes (4-7%). Environ Toxicol Chem 2019;38:321-328.
(c) 2018 SETAC.},
note = {ACL},
keywords = {ER4},
pubstate = {published},
tppubtype = {article}
}
We assessed the relationship between the diffusive gradient in thin
film (DGT) technique using the new ion-exchange resin Ambersep GT74
and the uptake of mercury (Hg) by a model plant cultivated on metal-contaminated
agricultural soils under greenhouse conditions. Based on the total
Hg content, 0.37 to 1.17% of the Hg passed to the soil porewater
from the solid phase, and 2.18 to 9.18% of the Hg is DGT-available.
These results were confirmed by calculating the R value (the ratio
of the concentrations of bioavailable Hg measured by DGT and soil
solution), which illustrated the strong bonding of Hg to the solid
phase of soil and its extremely low mobility. Only inorganic Hg(2+)
species were found in the metal-contaminated agricultural soils,
as determined by a high-performance liquid chromatography-cold vapor
atomic fluorescence spectrometry speciation analysis. The Hg was
distributed in Miscanthus x giganteus organs in the following order
for all sampling sites: roots (55-82%) >> leaves (8-27%) > stems
(7-16%) > rhizomes (4-7%). Environ Toxicol Chem 2019;38:321-328.
(c) 2018 SETAC. |
2019Conference ER4 Auteurs : Louzon, Maxime; Pauget, Benjamin; Pelfrêne, Aurélie; Gimbert, Frédéric; Crini, Nadia; Rieffel, Dominique; Amiot, Caroline; Douay, Francis; De-Vaufleury, Annette Couplage de la bioaccessibilité orale pour l’homme et de la biodisponibilité pour l’escargot 4ème Rencontres nationales de la Recherche sur les sites et sols pollués, Le Beffroi de Montrouge, 26-27 novembre 2019, Paris, 2019, (ACTN). Abstract @conference{Louzon2019c,
title = {Couplage de la bioaccessibilité orale pour l’homme et de la biodisponibilité pour l’escargot},
author = {Maxime Louzon and Benjamin Pauget and Aurélie Pelfrêne and Frédéric Gimbert and Nadia Crini and Dominique Rieffel and Caroline Amiot and Francis Douay and Annette De-Vaufleury},
year = {2019},
date = {2019-01-01},
booktitle = {4ème Rencontres nationales de la Recherche sur les sites et sols pollués, Le Beffroi de Montrouge, 26-27 novembre 2019, Paris},
abstract = {Dans le contexte de l’évaluation des risques sanitaires (ERS) et environnementaux
(ERE), un des objectifs du programme COMBINE, soutenu par l’ADEME
est de confronter les outils utilisés dans ces évaluations. Sur vingt-neuf
échantillons de terres contaminées par l’As, le Cd et le Pb, ont
été réalisées d’une part, un test in vitro de bioaccessibilité pour
l’homme (UBM) estimant la fraction des contaminants solubilisée au
niveau du tractus gastro-intestinal après ingestion de particules
de terre, et d’autre part, un test de bioaccumulation ex situ en
utilisant l’escargot. Les résultats montrent une influence des paramètres
physico-chimiques des terres sur la bioaccessibilité et la bioaccumulation
des contaminants par l’escargot. Les régressions multiples révèlent
de bonnes corrélations entre la bioaccumulation chez l’escargot et
la bioaccessibilité (r²adj entre 0,77 et 0,95) selon la nature et
la concentration du contaminant, des paramètres physico-chimiques
des terres, et de la phase gastrique ou gastro-intestinale du test
UBM. Pour les trois éléments métalliques étudiés, une forte relation
existe entre les méthodologies d’évaluation de la biodisponibilité
pour l’ERE et l’ERS. Ceci n’avait jamais encore été montré pour des
organismes présentant une physiologie et des modes d’exposition variés},
note = {ACTN},
keywords = {ER4},
pubstate = {published},
tppubtype = {conference}
}
Dans le contexte de l’évaluation des risques sanitaires (ERS) et environnementaux
(ERE), un des objectifs du programme COMBINE, soutenu par l’ADEME
est de confronter les outils utilisés dans ces évaluations. Sur vingt-neuf
échantillons de terres contaminées par l’As, le Cd et le Pb, ont
été réalisées d’une part, un test in vitro de bioaccessibilité pour
l’homme (UBM) estimant la fraction des contaminants solubilisée au
niveau du tractus gastro-intestinal après ingestion de particules
de terre, et d’autre part, un test de bioaccumulation ex situ en
utilisant l’escargot. Les résultats montrent une influence des paramètres
physico-chimiques des terres sur la bioaccessibilité et la bioaccumulation
des contaminants par l’escargot. Les régressions multiples révèlent
de bonnes corrélations entre la bioaccumulation chez l’escargot et
la bioaccessibilité (r²adj entre 0,77 et 0,95) selon la nature et
la concentration du contaminant, des paramètres physico-chimiques
des terres, et de la phase gastrique ou gastro-intestinale du test
UBM. Pour les trois éléments métalliques étudiés, une forte relation
existe entre les méthodologies d’évaluation de la biodisponibilité
pour l’ERE et l’ERS. Ceci n’avait jamais encore été montré pour des
organismes présentant une physiologie et des modes d’exposition variés |
2019Conference ER4 Auteurs : Pauget, Benjamin; Louzon, Maxime; Pelfrêne, Aurélie; Gimbert, Frédéric; Douay, Francis; De-Vaufleury, Annette Intégration de la biodisponibilité dans l’évaluation des risques sanitaires et environnementaux de sols contaminés 4ème Rencontres nationales de la Recherche sur les sites et sols pollués, Le Beffroi de Montrouge, 26-27 novembre 2019, Paris, 2019, (ACTN). @conference{Pauget2019,
title = {Intégration de la biodisponibilité dans l’évaluation des risques sanitaires et environnementaux de sols contaminés},
author = {Benjamin Pauget and Maxime Louzon and Aurélie Pelfrêne and Frédéric Gimbert and Francis Douay and Annette De-Vaufleury},
year = {2019},
date = {2019-01-01},
booktitle = {4ème Rencontres nationales de la Recherche sur les sites et sols pollués, Le Beffroi de Montrouge, 26-27 novembre 2019, Paris},
note = {ACTN},
keywords = {ER4},
pubstate = {published},
tppubtype = {conference}
}
|
2019Conference ER4 Auteurs : Pelfrêne, Aurélie; Le-Bot, Barbara; Waterlot, Christophe; Glorennec, Philippe; Sahmer, Karin; Douay, Francis Une méthode simplifiée pour estimer la bioaccessibilité des polluants métalliques dans les sols 4ème Rencontres nationales de la Recherche sur les sites et sols pollués, Le Beffroi de Montrouge, 26-27 novembre 2019, Paris, 2019, (ACTN). @conference{Pelfrene2019f,
title = {Une méthode simplifiée pour estimer la bioaccessibilité des polluants métalliques dans les sols},
author = {Aurélie Pelfrêne and Barbara Le-Bot and Christophe Waterlot and Philippe Glorennec and Karin Sahmer and Francis Douay},
year = {2019},
date = {2019-01-01},
booktitle = {4ème Rencontres nationales de la Recherche sur les sites et sols pollués, Le Beffroi de Montrouge, 26-27 novembre 2019, Paris},
note = {ACTN},
keywords = {ER4},
pubstate = {published},
tppubtype = {conference}
}
|
2018Conference ER4 Auteurs : Janus, Adeline; Pelfrêne, Aurélie; Bidar, Géraldine; Louvel, Brice; Douay, Francis Influence of two amendments on phyto- and sanitary availability of metals in highly contaminated soils: A greenhouse study International Conference Contaminated Sites 2018, 8-10 October 2018, Banská Bystrica (Slovak Republic), 2018, (COM). Abstract @conference{Janus2018,
title = {Influence of two amendments on phyto- and sanitary availability of metals in highly contaminated soils: A greenhouse study},
author = {Adeline Janus and Aurélie Pelfrêne and Géraldine Bidar and Brice Louvel and Francis Douay},
year = {2018},
date = {2018-01-01},
booktitle = {International Conference Contaminated Sites 2018, 8-10 October 2018, Banská Bystrica (Slovak Republic)},
pages = {101},
abstract = {Soil is an essential and non-renewable resource which can perform
a high number of economic, social and environmental functions as
biomass production, source of raw materials or protection of humans
and environment (Blum, 2005). However, the soil functionality becomes
increasingly compromised due to contaminations caused by human activities.
In 2006 and in 39 countries, the European Environmental Agency inventoried
approximately 3 million of sites where pollutant activities occurred
with more than 1 .8 million potentially contaminated sites (CGDD
2013). In 2012, the most frequently identified contaminants were
metals (35 %), hydrocarbons (24 %) and polycyclic aromatic hydrocarbons
(11 %). Until recently, the most common remediation technique was
the excavation of contaminated soil and its disposal as landfill.
However, this kind of method is considered inappropriate because
it generates considerable disturbances, is expensive and economically
unfeasible on a large scale . Thus, other remediation techniques
(ex and in situ) have been developed to overcome these disadvantages
. Among them, a technique consists in adding inorganic or organic
amendments to the contaminated soils in order to decrease the mobility
and bioavailability of pollutants in soils (Kumpiene et al., 2008;
Vangronsveld et al., 2009; Bolan et al., 2014; Nejad et al., 2017)
. The most often used amendments are phosphate compounds, liming
materials, metal oxides and biochars, used alone or in combination
(Waterlot et al., 2017; Lahori et al., 2017; Oustrière et al., 2017).
The goal of the present work consists in evaluating the ability of
two amendments (woody biochar and iron grit, used alone or in combination)
to immobilize Cd, Cu, Pb, and Zn in contaminated soils under greenhouse
conditions},
note = {COM},
keywords = {ER4},
pubstate = {published},
tppubtype = {conference}
}
Soil is an essential and non-renewable resource which can perform
a high number of economic, social and environmental functions as
biomass production, source of raw materials or protection of humans
and environment (Blum, 2005). However, the soil functionality becomes
increasingly compromised due to contaminations caused by human activities.
In 2006 and in 39 countries, the European Environmental Agency inventoried
approximately 3 million of sites where pollutant activities occurred
with more than 1 .8 million potentially contaminated sites (CGDD
2013). In 2012, the most frequently identified contaminants were
metals (35 %), hydrocarbons (24 %) and polycyclic aromatic hydrocarbons
(11 %). Until recently, the most common remediation technique was
the excavation of contaminated soil and its disposal as landfill.
However, this kind of method is considered inappropriate because
it generates considerable disturbances, is expensive and economically
unfeasible on a large scale . Thus, other remediation techniques
(ex and in situ) have been developed to overcome these disadvantages
. Among them, a technique consists in adding inorganic or organic
amendments to the contaminated soils in order to decrease the mobility
and bioavailability of pollutants in soils (Kumpiene et al., 2008;
Vangronsveld et al., 2009; Bolan et al., 2014; Nejad et al., 2017)
. The most often used amendments are phosphate compounds, liming
materials, metal oxides and biochars, used alone or in combination
(Waterlot et al., 2017; Lahori et al., 2017; Oustrière et al., 2017).
The goal of the present work consists in evaluating the ability of
two amendments (woody biochar and iron grit, used alone or in combination)
to immobilize Cd, Cu, Pb, and Zn in contaminated soils under greenhouse
conditions |
2018Conference ER4 Auteurs : Nguyen, Van-Xuan; Douay, Francis; Alary, Claire; Mamindy-Pajany, Yannick; Pelfrêne, Aurélie Caractérisation de la disponibilité environnementale et toxicologique de Cd et Pb dans des anthroposols issus de sédiments de dragage fluviaux International Conference Contaminated Sites 2018, 8-10 October 2018, Banská Bystrica (Slovak Republic), 2018, (COM). @conference{Nguyen2018,
title = {Caractérisation de la disponibilité environnementale et toxicologique de Cd et Pb dans des anthroposols issus de sédiments de dragage fluviaux},
author = {Van-Xuan Nguyen and Francis Douay and Claire Alary and Yannick Mamindy-Pajany and Aurélie Pelfrêne},
year = {2018},
date = {2018-01-01},
booktitle = {International Conference Contaminated Sites 2018, 8-10 October 2018, Banská Bystrica (Slovak Republic)},
note = {COM},
keywords = {ER4},
pubstate = {published},
tppubtype = {conference}
}
|
2018Conference ER4 Auteurs : Nguyen, Van-Xuan; Douay, Francis; Mamindy-Pajany, Yannick; Alary, Claire; Pelfrêne, Aurélie Caractérisation de la disponibilité environnementale et toxicologique de Cd et Pb dans des anthroposols issus de sédiments de dragage fluviaux 26e Réunion des Sciences de la Terre, 22-26 octobre 2018, Lille, 2018, (ACTN). @conference{Nguyen2018a,
title = {Caractérisation de la disponibilité environnementale et toxicologique de Cd et Pb dans des anthroposols issus de sédiments de dragage fluviaux},
author = {Van-Xuan Nguyen and Francis Douay and Yannick Mamindy-Pajany and Claire Alary and Aurélie Pelfrêne},
year = {2018},
date = {2018-01-01},
booktitle = {26e Réunion des Sciences de la Terre, 22-26 octobre 2018, Lille},
note = {ACTN},
keywords = {ER4},
pubstate = {published},
tppubtype = {conference}
}
|
2018Conference ER4 Auteurs : Nguyen, Van-Xuan; Douay, Francis; Mamindy-Pajany, Yannick; Alary, Claire; Pelfrêne, Aurélie Importance of environmental and toxicological availabilities of Cd and Pb in management of dredged sediments International Conference Contaminated Sites 2018, 8-10 October 2018, Banská Bystrica (Slovak Republic), 2018, (COM). @conference{Nguyen2018b,
title = {Importance of environmental and toxicological availabilities of Cd and Pb in management of dredged sediments},
author = {Van-Xuan Nguyen and Francis Douay and Yannick Mamindy-Pajany and Claire Alary and Aurélie Pelfrêne},
year = {2018},
date = {2018-01-01},
booktitle = {International Conference Contaminated Sites 2018, 8-10 October 2018, Banská Bystrica (Slovak Republic)},
note = {COM},
keywords = {ER4},
pubstate = {published},
tppubtype = {conference}
}
|
2018Conference ER4 Auteurs : Sahmer, Karin; Potel, A; Waterlot, Christophe; Pelfrêne, Aurélie Modélisation de l’accumulation du cadmium dans des légumes en fonction des concentrations extractibles des sols Chimiométrie XIX, 30-31 janvier 2018, Paris, 2018, (AFF). @conference{Sahmer2018,
title = {Modélisation de l’accumulation du cadmium dans des légumes en fonction des concentrations extractibles des sols},
author = {Karin Sahmer and A Potel and Christophe Waterlot and Aurélie Pelfrêne},
year = {2018},
date = {2018-01-01},
booktitle = {Chimiométrie XIX, 30-31 janvier 2018, Paris},
note = {AFF},
keywords = {ER4},
pubstate = {published},
tppubtype = {conference}
}
|
2018Journal Article ER4 Auteurs : Pelfrêne, Aurélie; Douay, Francis Assessment of oral and lung bioaccessibility of Cd and Pb from smelter-impacted dust In: Environmental Science and Pollution Research, vol. 25, no. 4, pp. 3718-3730, 2018, (ACL). Abstract @article{Pelfrene2018,
title = {Assessment of oral and lung bioaccessibility of Cd and Pb from smelter-impacted dust},
author = {Aurélie Pelfrêne and Francis Douay},
year = {2018},
date = {2018-01-01},
journal = {Environmental Science and Pollution Research},
volume = {25},
number = {4},
pages = {3718-3730},
abstract = {Soil and dust contamination by metals engenders significant environmental
and health problems in northern France where a lead smelter was in
activity for more than a century. This study aims to examine the
long-term effects of the smelter, 10 years after its closedown, on
the presence of metal in sidewalk dust for a better assessment of
the local population's exposure to Cd and Pb. The investigation included:
(i) the metal distribution in different dust particle sizes and (ii)
the assessment of metal bioaccessibility via ingestion and inhalation
of dust. Seventy-two sidewalk dust samples were collected using a
dust-sampling vacuum. The samples were sieved to collect different
particle sizes from 0.3 to 1000 mu m. The unified bioaccessibility
method (UBM) was employed to evaluate the oral bioaccessibility of
metals in the different particle sizes. The pulmonary bioaccessible
fraction of Cd and Pb via the finest particles was extracted with
lung-simulating solution (artificial lysosomal fluid). Ten years
after the smelter closedown, (i) a strong relationship was observed
between the concentrations of metals in dust and the distance to
the former smelter, whatever the particle size; (ii) both total and
oral bioaccessible concentrations of metals were high in the finest
fraction (0.3-5 mu m) and decreased when the particle size increased;
(iii) a higher oral bioaccessibility of Cd and Pb was measured in
the gastric phase (on average 43% for both metals for all particle
sizes) and compared to the gastrointestinal phase (on average 16%
for both metals for all particle sizes); and (iv) metal bioaccessibility
via inhalation of dust was relatively high (on average 74 and 69%,
for Cd and Pb, respectively). The results of the present study suggest
that this environmental compartment may be a sensitive and effective
indicator of anthropogenic metal contamination and the human exposure
in urban areas.},
note = {ACL},
keywords = {ER4},
pubstate = {published},
tppubtype = {article}
}
Soil and dust contamination by metals engenders significant environmental
and health problems in northern France where a lead smelter was in
activity for more than a century. This study aims to examine the
long-term effects of the smelter, 10 years after its closedown, on
the presence of metal in sidewalk dust for a better assessment of
the local population's exposure to Cd and Pb. The investigation included:
(i) the metal distribution in different dust particle sizes and (ii)
the assessment of metal bioaccessibility via ingestion and inhalation
of dust. Seventy-two sidewalk dust samples were collected using a
dust-sampling vacuum. The samples were sieved to collect different
particle sizes from 0.3 to 1000 mu m. The unified bioaccessibility
method (UBM) was employed to evaluate the oral bioaccessibility of
metals in the different particle sizes. The pulmonary bioaccessible
fraction of Cd and Pb via the finest particles was extracted with
lung-simulating solution (artificial lysosomal fluid). Ten years
after the smelter closedown, (i) a strong relationship was observed
between the concentrations of metals in dust and the distance to
the former smelter, whatever the particle size; (ii) both total and
oral bioaccessible concentrations of metals were high in the finest
fraction (0.3-5 mu m) and decreased when the particle size increased;
(iii) a higher oral bioaccessibility of Cd and Pb was measured in
the gastric phase (on average 43% for both metals for all particle
sizes) and compared to the gastrointestinal phase (on average 16%
for both metals for all particle sizes); and (iv) metal bioaccessibility
via inhalation of dust was relatively high (on average 74 and 69%,
for Cd and Pb, respectively). The results of the present study suggest
that this environmental compartment may be a sensitive and effective
indicator of anthropogenic metal contamination and the human exposure
in urban areas. |
2018Journal Article ER4 Auteurs : Janus, Adeline; Waterlot, Christophe; Heymans, Sophie; Deboffe, Christophe; Douay, Francis; Pelfrêne, Aurélie Do biochars influence the availability and human oral bioaccessibility of Cd, Pb, and Zn in a contaminated slightly alkaline soil? In: Environmental Monitoring and Assessment, vol. 190, no. 218, pp. 1-13, 2018, (ACL). Abstract @article{Janus2018b,
title = {Do biochars influence the availability and human oral bioaccessibility of Cd, Pb, and Zn in a contaminated slightly alkaline soil?},
author = {Adeline Janus and Christophe Waterlot and Sophie Heymans and Christophe Deboffe and Francis Douay and Aurélie Pelfrêne},
year = {2018},
date = {2018-01-01},
journal = {Environmental Monitoring and Assessment},
volume = {190},
number = {218},
pages = {1-13},
abstract = {Different remediation techniques have been used to restore metal-contaminated
sites, including stabilizing metals by adding amendments to the soils.
This study experimented three biochars, made from wood and miscanthus,
cultivated on contaminated and uncontaminated soils, used as amendments
at a 2% application rate on a metal-contaminated soil for 9 months
in laboratory-controlled conditions. The objective was to evaluate
whether biochars were able to decrease the availability and human
oral bioaccessibility of metals in an alkaline soil. To meet this
goal, the modifications of the soil’s physicochemical parameters,
metal distribution in soil, and human bioaccessibility were evaluated
at different sampling times. The results showed that biochar application
to the alkaline soil did not always decrease the soil metal availability,
which challenges the value of using biochars in already slightly
alkaline soils at a low application rate. However, differences in
efficiency between the three biochars tested were highlighted. The
biochar produced with miscanthus cultivated on uncontaminated soil
led to higher soil metal bioaccessibility. Moreover, because of the
absence of any increase in soil metal availability with the biochar
produced from biomass cultivated on contaminated soil, the use of
such biochars can be recommended for the remediation of contaminated
soil.},
note = {ACL},
keywords = {ER4},
pubstate = {published},
tppubtype = {article}
}
Different remediation techniques have been used to restore metal-contaminated
sites, including stabilizing metals by adding amendments to the soils.
This study experimented three biochars, made from wood and miscanthus,
cultivated on contaminated and uncontaminated soils, used as amendments
at a 2% application rate on a metal-contaminated soil for 9 months
in laboratory-controlled conditions. The objective was to evaluate
whether biochars were able to decrease the availability and human
oral bioaccessibility of metals in an alkaline soil. To meet this
goal, the modifications of the soil’s physicochemical parameters,
metal distribution in soil, and human bioaccessibility were evaluated
at different sampling times. The results showed that biochar application
to the alkaline soil did not always decrease the soil metal availability,
which challenges the value of using biochars in already slightly
alkaline soils at a low application rate. However, differences in
efficiency between the three biochars tested were highlighted. The
biochar produced with miscanthus cultivated on uncontaminated soil
led to higher soil metal bioaccessibility. Moreover, because of the
absence of any increase in soil metal availability with the biochar
produced from biomass cultivated on contaminated soil, the use of
such biochars can be recommended for the remediation of contaminated
soil. |
2017Conference ER4 Auteurs : Douay, Francis; Lefebvre, Gaëtan; Branchu, Philippe; Pelfrêne, Aurélie; Lebeau, Thierry; Rémy, Elisabeth Jardins collectifs urbains et contaminations des sols : retours d’expérience sur l’évaluation des risques sanitaires International congress - Sustainable Urban Agricultures: Vector for the Ecological Transition, 6-9 juin 2017, Toulouse, 2017, (ACTI). Abstract @conference{Douay2017,
title = {Jardins collectifs urbains et contaminations des sols : retours d’expérience sur l’évaluation des risques sanitaires},
author = {Francis Douay and Gaëtan Lefebvre and Philippe Branchu and Aurélie Pelfrêne and Thierry Lebeau and Elisabeth Rémy},
year = {2017},
date = {2017-01-01},
booktitle = {International congress - Sustainable Urban Agricultures: Vector for the Ecological Transition, 6-9 juin 2017, Toulouse},
abstract = {Avec la montée en puissance de préoccupations en lien avec l’environnement et le « manger sain », on constate une demande croissante pour les jardins collectifs urbains (jardins familiaux, partagés, pédagogiques ou encore d’insertion) (canavese, 2014). cependant, résultant de processus géologiques et pédologiques hétérogènes (pouvant dans certains cas être à l’origine d’anomalies avec fortes concentrations en certains éléments métalliques, cf. jean-soro et al. 2014; bouquet et al., 2016), leurs sols sont des milieux très complexes et réactifs aux activités humaines et industrielles (douay, 2008). les jardins collectifs présentent la particularité d’être très souvent en milieu urbain ou périurbain et leurs sols ont été fréquemment remaniés, d’où la difficulté de retracer l’historique et, parfois, l’origine des contaminants. de fait, les jardins sont souvent aménagés sur des espaces qui ont été exposés par le passé à une, voire plusieurs sources de contamination. à ce jour, demeurent de nombreuses sources de contaminations (potentielles ou avérées) telles que la proximité d’industries, d’axes routiers ou ferroviaires susceptibles d’impacter la qualité de ces milieux comme supports de cultures, l'utilisation fréquente de produits phytosanitaires (même lorsque la charte du jardin ou de la ville l’interdit) qui peuvent conduire à modifier le fonctionnement du sol, ou encore l’utilisation pour l’irrigation d’eau contaminée. à cela s’ajoutent les sources de contaminations urbaines issues de la circulation automobile, du chauffage et de l’altération des constructions et des matériaux. dans ce contexte, les jardins peuvent présenter un risque du fait d’une contamination de leurs sols et plus globalement du milieu où ils sont localisés, surtout lorsqu’ils concernent une population dite « sensible » (enfants, femmes enceintes, personnes âgées). l’exposition aux polluants peut être liée à la consommation de légumes et/ou à l’inhalation ou à l’ingestion de particules de terre contaminées. une autre voie d’exposition est celle de la pollution atmosphérique dont les effets sont accentués par l’activité physique associée au jardinage. d’un point de vue réglementaire et contrairement à l’air ou à l’eau, le sol a un statut très particulier puisqu’il n’est pas protégé en tant que tel. l’absence de valeurs seuils réglementant les usages des sols pèse sur la gestion des jardins urbains, espaces récréatifs et de productions alimentaires. en cas de contamination environnementale avérée, la démarche nationale repose sur les procédures réglementaires d’évaluation de risques sanitaires des sites et sols pollués. dans le cadre d’une démarche pluridisciplinaire, il a été décidé de centrer notre attention sur l’outil « evaluation quantitative des risques sanitaires –eqrs » préconisé dans le cadre de la méthodologie nationale et appliqué à la problématique des jardins associatifs. après un rappel des étapes relatives à cet outil, seront exposés les contextes et les démarches de cinq études réalisées sur des jardins familiaux français situés dans différents contextes environnementaux. le retour d’expérience sur l’analyse des eqrs étudiées a mis en évidence six points majeurs, lesquels seront présentés et discutés : - les compétences du maître d’ouvrage / maître d’oeuvre pour définir ce qui est à faire ou à ne pas faire dans le cadre d’une eqrs ; - les données nécessaires pour la réalisation d’une eqrs en soulignant l’importance du diagnostic historique ; - les incertitudes liées à la mesure des concentrations en polluants dans les matrices échantillonnées ; - les difficultés qui résultent de l’absence de valeurs réglementaires pour déclarer qu’un sol est contaminé et du recours à des référentiels plus ou moins adaptés au contexte et aux objectifs de la démarche ; - les incertitudes sur les paramètres à considérer dans l’eqrs (quantités de particules de terre et de légumes ingérés, part des légumes autoproduits…) ; - la perception du sol par les jardiniers et la nécessité de définir un langage commun pour ne pas générer de problèmes d’interprétation et répondre aux questions que se posent ces acteurs. l’analyse des cinq exemples d’eqrs atteste l’importance des paramètres à considérer pour une telle démarche. le présent travail représente un apport méthodologique en vue d’essayer de guider les pratiques et aussi, de répondre aux collectivités, lesquelles sont de plus en plus confrontées à des problèmes de contamination des sols de jardin et veulent s’engager dans la réalisation d’une eqrs. au vu de certains résultats, des jardiniers vont se documenter, chercher des réponses auprès des mairies, des bureaux d’études, de l’ars, de scientifiques… l’expérience souligne aussi l’absence de référent qui pourrait renseigner sur la qualité des sols et de leur gestion en milieu contaminé. la restitution des résultats auprès des gestionnaires de jardins et des populations concernées nécessite une réflexion approfondie associant les parties concernées et des spécialistes de la santé.},
note = {ACTI},
keywords = {ER4},
pubstate = {published},
tppubtype = {conference}
}
Avec la montée en puissance de préoccupations en lien avec l’environnement et le « manger sain », on constate une demande croissante pour les jardins collectifs urbains (jardins familiaux, partagés, pédagogiques ou encore d’insertion) (canavese, 2014). cependant, résultant de processus géologiques et pédologiques hétérogènes (pouvant dans certains cas être à l’origine d’anomalies avec fortes concentrations en certains éléments métalliques, cf. jean-soro et al. 2014; bouquet et al., 2016), leurs sols sont des milieux très complexes et réactifs aux activités humaines et industrielles (douay, 2008). les jardins collectifs présentent la particularité d’être très souvent en milieu urbain ou périurbain et leurs sols ont été fréquemment remaniés, d’où la difficulté de retracer l’historique et, parfois, l’origine des contaminants. de fait, les jardins sont souvent aménagés sur des espaces qui ont été exposés par le passé à une, voire plusieurs sources de contamination. à ce jour, demeurent de nombreuses sources de contaminations (potentielles ou avérées) telles que la proximité d’industries, d’axes routiers ou ferroviaires susceptibles d’impacter la qualité de ces milieux comme supports de cultures, l'utilisation fréquente de produits phytosanitaires (même lorsque la charte du jardin ou de la ville l’interdit) qui peuvent conduire à modifier le fonctionnement du sol, ou encore l’utilisation pour l’irrigation d’eau contaminée. à cela s’ajoutent les sources de contaminations urbaines issues de la circulation automobile, du chauffage et de l’altération des constructions et des matériaux. dans ce contexte, les jardins peuvent présenter un risque du fait d’une contamination de leurs sols et plus globalement du milieu où ils sont localisés, surtout lorsqu’ils concernent une population dite « sensible » (enfants, femmes enceintes, personnes âgées). l’exposition aux polluants peut être liée à la consommation de légumes et/ou à l’inhalation ou à l’ingestion de particules de terre contaminées. une autre voie d’exposition est celle de la pollution atmosphérique dont les effets sont accentués par l’activité physique associée au jardinage. d’un point de vue réglementaire et contrairement à l’air ou à l’eau, le sol a un statut très particulier puisqu’il n’est pas protégé en tant que tel. l’absence de valeurs seuils réglementant les usages des sols pèse sur la gestion des jardins urbains, espaces récréatifs et de productions alimentaires. en cas de contamination environnementale avérée, la démarche nationale repose sur les procédures réglementaires d’évaluation de risques sanitaires des sites et sols pollués. dans le cadre d’une démarche pluridisciplinaire, il a été décidé de centrer notre attention sur l’outil « evaluation quantitative des risques sanitaires –eqrs » préconisé dans le cadre de la méthodologie nationale et appliqué à la problématique des jardins associatifs. après un rappel des étapes relatives à cet outil, seront exposés les contextes et les démarches de cinq études réalisées sur des jardins familiaux français situés dans différents contextes environnementaux. le retour d’expérience sur l’analyse des eqrs étudiées a mis en évidence six points majeurs, lesquels seront présentés et discutés : - les compétences du maître d’ouvrage / maître d’oeuvre pour définir ce qui est à faire ou à ne pas faire dans le cadre d’une eqrs ; - les données nécessaires pour la réalisation d’une eqrs en soulignant l’importance du diagnostic historique ; - les incertitudes liées à la mesure des concentrations en polluants dans les matrices échantillonnées ; - les difficultés qui résultent de l’absence de valeurs réglementaires pour déclarer qu’un sol est contaminé et du recours à des référentiels plus ou moins adaptés au contexte et aux objectifs de la démarche ; - les incertitudes sur les paramètres à considérer dans l’eqrs (quantités de particules de terre et de légumes ingérés, part des légumes autoproduits…) ; - la perception du sol par les jardiniers et la nécessité de définir un langage commun pour ne pas générer de problèmes d’interprétation et répondre aux questions que se posent ces acteurs. l’analyse des cinq exemples d’eqrs atteste l’importance des paramètres à considérer pour une telle démarche. le présent travail représente un apport méthodologique en vue d’essayer de guider les pratiques et aussi, de répondre aux collectivités, lesquelles sont de plus en plus confrontées à des problèmes de contamination des sols de jardin et veulent s’engager dans la réalisation d’une eqrs. au vu de certains résultats, des jardiniers vont se documenter, chercher des réponses auprès des mairies, des bureaux d’études, de l’ars, de scientifiques… l’expérience souligne aussi l’absence de référent qui pourrait renseigner sur la qualité des sols et de leur gestion en milieu contaminé. la restitution des résultats auprès des gestionnaires de jardins et des populations concernées nécessite une réflexion approfondie associant les parties concernées et des spécialistes de la santé. |
2017Conference ER4 Auteurs : Dumat, Camille; Pelfrêne, Aurélie; Lévêque, Thibaut; Mombo, Stéphane; Austruy, Annabelle; Shins, R; Foucault, Yann Measurement of human bioaccessibility for metals: Relevant indicator of the link environment-health! International congress - Sustainable Urban Agricultures: Vector for the Ecological Transition, 6-9 juin 2017, Toulouse, 2017, (AFF). @conference{Dumat2017,
title = {Measurement of human bioaccessibility for metals: Relevant indicator of the link environment-health!},
author = {Camille Dumat and Aurélie Pelfrêne and Thibaut Lévêque and Stéphane Mombo and Annabelle Austruy and R Shins and Yann Foucault},
year = {2017},
date = {2017-01-01},
booktitle = {International congress - Sustainable Urban Agricultures: Vector for the Ecological Transition, 6-9 juin 2017, Toulouse},
note = {AFF},
keywords = {ER4},
pubstate = {published},
tppubtype = {conference}
}
|
2017Journal Article ER4 Auteurs : Janus, Adeline; Goulas, Anaïs; Pelfrêne, Aurélie; Douay, Francis; Waterlot, Christophe Determination of PAHs by ultra fast liquid chromatography using a coreshell technology – Application to their determination after using biochar as adsorbent In: Measurement, vol. 106, pp. 137-142, 2017, (ACL). Abstract @article{Janus2017a,
title = {Determination of PAHs by ultra fast liquid chromatography using a coreshell technology – Application to their determination after using biochar as adsorbent},
author = {Adeline Janus and Anaïs Goulas and Aurélie Pelfrêne and Francis Douay and Christophe Waterlot},
year = {2017},
date = {2017-01-01},
journal = {Measurement},
volume = {106},
pages = {137-142},
abstract = {The c18 column (250 mm 4.6 mm) packed with 5 lm core-shell particles was used in an effort to optimize the separation of 8 polycyclic aromatic hydrocarbons under very low pressure values (44–52 bars), low temperature (16 c) and in 13 min. chromatogram and peaks of each polycyclic aromatic hydrocarbon studied, obtained using an ultra fast liquid chromatography fitted with this column and equipped with a diode array detector, were compared with those obtained using two other traditional c18 columns, packed with fully porous 5 lm particles, usually used in our laboratory and specifically designed for the separation of polycyclic aromatic hydrocarbons. thinnest peaks, highest sensitivity and efficiency are the main results related to the core-shell technology of the recent kinetex column compared to more common c18 columns due to the bed uniformity and packing quality of the recent core-shell column. on the other hand, reduced retention time was highlighted for each polycyclic aromatic hydrocarbon using the column packed with core-shell particles resulting from the lower surface area of these particles compared to the totally porous particles of the both other columns used. limits of detection and quantification, linearity range and repeatability were determined for the method developed with the core-shell column. a practical application was realized by evaluating the sorption capacity of the 8 polycyclic aromatic hydrocarbons studied in mixture using a biochar made from woody plants. to this end, the biochar was mixed with aqueous solution spiked with the mixture of polycyclic aromatic hydrocarbons and a kinetic study of their sorption was conducted. sorption percentage was higher than 89% for each polycyclic aromatic hydrocarbon studied showing that the studied biochar could be good and low cost alternative products for the sorption of this type of pollutants.},
note = {ACL},
keywords = {ER4},
pubstate = {published},
tppubtype = {article}
}
The c18 column (250 mm 4.6 mm) packed with 5 lm core-shell particles was used in an effort to optimize the separation of 8 polycyclic aromatic hydrocarbons under very low pressure values (44–52 bars), low temperature (16 c) and in 13 min. chromatogram and peaks of each polycyclic aromatic hydrocarbon studied, obtained using an ultra fast liquid chromatography fitted with this column and equipped with a diode array detector, were compared with those obtained using two other traditional c18 columns, packed with fully porous 5 lm particles, usually used in our laboratory and specifically designed for the separation of polycyclic aromatic hydrocarbons. thinnest peaks, highest sensitivity and efficiency are the main results related to the core-shell technology of the recent kinetex column compared to more common c18 columns due to the bed uniformity and packing quality of the recent core-shell column. on the other hand, reduced retention time was highlighted for each polycyclic aromatic hydrocarbon using the column packed with core-shell particles resulting from the lower surface area of these particles compared to the totally porous particles of the both other columns used. limits of detection and quantification, linearity range and repeatability were determined for the method developed with the core-shell column. a practical application was realized by evaluating the sorption capacity of the 8 polycyclic aromatic hydrocarbons studied in mixture using a biochar made from woody plants. to this end, the biochar was mixed with aqueous solution spiked with the mixture of polycyclic aromatic hydrocarbons and a kinetic study of their sorption was conducted. sorption percentage was higher than 89% for each polycyclic aromatic hydrocarbon studied showing that the studied biochar could be good and low cost alternative products for the sorption of this type of pollutants. |
2017Journal Article ER4 Auteurs : Janus, Adeline; Pelfrêne, Aurélie; Sahmer, Karin; Heymans, Sophie; Deboffe, Christophe; Douay, Francis; Waterlot, Christophe Value of biochars from Miscanthus x giganteus cultivated on contaminated soils to decrease the availability of metals in multicontaminated aqueous solutions In: Environmental Science and Pollution Research, vol. 24, no. 22, pp. 18204-18217, 2017, (ACL). Abstract @article{Janus2017b,
title = {Value of biochars from Miscanthus x giganteus cultivated on contaminated soils to decrease the availability of metals in multicontaminated aqueous solutions},
author = {Adeline Janus and Aurélie Pelfrêne and Karin Sahmer and Sophie Heymans and Christophe Deboffe and Francis Douay and Christophe Waterlot},
year = {2017},
date = {2017-01-01},
journal = {Environmental Science and Pollution Research},
volume = {24},
number = {22},
pages = {18204-18217},
abstract = {The objective of this study was to evaluate the sorption efficiency of eight biochars, made from miscanthus x giganteus cultivated on contaminated agricultural soil, in aqueous solutions contaminated with metals alone or mixed with polycyclic aromatic hydrocarbons. these biochars were produced in different pyrolysis conditions (temperature, 400/600 °c; heating rate, 5/10 °c min−1; duration, 45/90 min) and compared with an uncontaminated commercialized biochar made of wood. the physicochemical characterization of the miscanthus biochars confirmed the impact of the pyrolysis on the biochar parameters with substantial differences between the biochars in terms of ph, cation exchange capacity, and specific surface area. the sorption experiment showed higher sorption efficiency of cd, pb, and zn for the miscanthus biochars produced at 600 °c compared with the biochars produced at 400 °c when the aqueous solutions were mono- or multicontaminated. furthermore, the desorption study showed that the sorption process was largely irreversible. therefore, the high sorption capacity of miscanthus biochars and the low sorption reversibility confirmed that these biochars are a suitable sorbent for metals.},
note = {ACL},
keywords = {ER4},
pubstate = {published},
tppubtype = {article}
}
The objective of this study was to evaluate the sorption efficiency of eight biochars, made from miscanthus x giganteus cultivated on contaminated agricultural soil, in aqueous solutions contaminated with metals alone or mixed with polycyclic aromatic hydrocarbons. these biochars were produced in different pyrolysis conditions (temperature, 400/600 °c; heating rate, 5/10 °c min−1; duration, 45/90 min) and compared with an uncontaminated commercialized biochar made of wood. the physicochemical characterization of the miscanthus biochars confirmed the impact of the pyrolysis on the biochar parameters with substantial differences between the biochars in terms of ph, cation exchange capacity, and specific surface area. the sorption experiment showed higher sorption efficiency of cd, pb, and zn for the miscanthus biochars produced at 600 °c compared with the biochars produced at 400 °c when the aqueous solutions were mono- or multicontaminated. furthermore, the desorption study showed that the sorption process was largely irreversible. therefore, the high sorption capacity of miscanthus biochars and the low sorption reversibility confirmed that these biochars are a suitable sorbent for metals. |
2017Conference ER4 Auteurs : Pelfrêne, Aurélie Projet ODESSA: Amélioration de l’évaluation des risques encourus par les populations exposées aux sols pollués en proposant une méthode alternative au test UBM, rapide, moins coûteuse, fiable, représentative de la bioaccessibilité gastro-intestinale des ETM et applicable dans différents contextes environnementaux Colloque ADEME Sites et Sols pollués, 10-11 mai 2017, Paris, 2017, (ACTN). @conference{Pelfrene2017a,
title = {Projet ODESSA: Amélioration de l’évaluation des risques encourus par les populations exposées aux sols pollués en proposant une méthode alternative au test UBM, rapide, moins coûteuse, fiable, représentative de la bioaccessibilité gastro-intestinale des ETM et applicable dans différents contextes environnementaux},
author = {Aurélie Pelfrêne},
year = {2017},
date = {2017-01-01},
booktitle = {Colloque ADEME Sites et Sols pollués, 10-11 mai 2017, Paris},
note = {ACTN},
keywords = {ER4},
pubstate = {published},
tppubtype = {conference}
}
|
2017Journal Article ER4 Auteurs : Pelfrêne, Aurélie; Cave, Mark-R.; Wragg, Joanna; Douay, Francis In vitro investigations of human bioaccessibility from reference materials using simulated lung fluids In: International Journal of Environmental Research and Public Health, vol. 14, no. 2, pp. 112, 2017, (ACL). Abstract @article{Pelfrene2017b,
title = {In vitro investigations of human bioaccessibility from reference materials using simulated lung fluids},
author = {Aurélie Pelfrêne and Mark-R. Cave and Joanna Wragg and Francis Douay},
year = {2017},
date = {2017-01-01},
journal = {International Journal of Environmental Research and Public Health},
volume = {14},
number = {2},
pages = {112},
abstract = {An investigation for assessing pulmonary bioaccessibility of metals from reference materials is presented using simulated lung fluids. the objective of this paper was to contribute to an enhanced understanding of airborne particulate matter and its toxic potential following inhalation. a large set of metallic elements (ba, cd, co, cr, cu, mn, ni, pb, sr, and zn) was investigated using three lung fluids (phosphate-buffered saline, gamble’s solution and artificial lysosomal fluid) on three standard reference materials representing different types of particle sources. composition of the leaching solution and four solid-to-liquid (s/l) ratios were tested. the results showed that bioaccessibility was speciation- (i.e., distribution) and element-dependent, with percentages varying from 0.04% for pb to 86.0% for cd. the higher extraction of metallic elements was obtained with the artificial lysosomal fluid, in which a relative stability of bioaccessibility was observed in a large range of s/l ratios from 1/1000 to 1/10,000. for further investigations, it is suggested that this method be used to assess lung bioaccessibility of metals from smelter-impacted dusts.},
note = {ACL},
keywords = {ER4},
pubstate = {published},
tppubtype = {article}
}
An investigation for assessing pulmonary bioaccessibility of metals from reference materials is presented using simulated lung fluids. the objective of this paper was to contribute to an enhanced understanding of airborne particulate matter and its toxic potential following inhalation. a large set of metallic elements (ba, cd, co, cr, cu, mn, ni, pb, sr, and zn) was investigated using three lung fluids (phosphate-buffered saline, gamble’s solution and artificial lysosomal fluid) on three standard reference materials representing different types of particle sources. composition of the leaching solution and four solid-to-liquid (s/l) ratios were tested. the results showed that bioaccessibility was speciation- (i.e., distribution) and element-dependent, with percentages varying from 0.04% for pb to 86.0% for cd. the higher extraction of metallic elements was obtained with the artificial lysosomal fluid, in which a relative stability of bioaccessibility was observed in a large range of s/l ratios from 1/1000 to 1/10,000. for further investigations, it is suggested that this method be used to assess lung bioaccessibility of metals from smelter-impacted dusts. |
